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Biomass-derived porous activated carbon nanofibers from Sapindus trifoliatus nut shells for high-performance symmetric supercapacitor applications
Carbon Letters ( IF 5.5 ) Pub Date : 2021-03-01 , DOI: 10.1007/s42823-021-00235-4
Murugan Vinayagam , Rajendran Suresh Babu , Arumugam Sivasamy , Ana Lucia Ferreira de Barros

Cost-effective and sustainable high-performance supercapacitor material was successfully prepared from cellulosic waste (Sapindus trifoliatus nut shells) biomass-derived activated carbon (CBAC) by physical activation method. The CBAC displays nanofiber morphology, high specific surface area (786 m2/g), large pore volume (0.212 cm3 g−1) which are evaluated using FESEM, BET and possessed excellent electrochemical behavior analyzed through various electrochemical methods. Moreover, the assembled symmetric CBAC//CBAC device exhibits high specific capacitance of 240.8 F g−1 with current density of 0.2 A g−1 and it is maintained to 65.6 F g−1 at high current density of 2.0 A g−1. In addition, the symmetric device delivers an excellent specific energy maximum of over 30 Wh kg−1 at 400 W kg−1 of specific power and excellent cycling stability in long term over 5000 cycles. The operation of the device was tested by light-emitting diode. Hence, CBAC-based materials pave way for developing large-scale, low-cost materials for energy storage device applications.



中文翻译:

Sapindus trifoliatus坚果壳的生物质多孔活性炭纳米纤维,用于高性能对称超级电容器应用

通过物理活化法成功地从纤维素废料(壳果坚果壳)生物质衍生的活性炭(CBAC)中制备了具有成本效益和可持续发展的高性能超级电容器材料。CBAC表现出纳米纤维形态,高比表面积(786 m 2 / g),大孔体积(0.212 cm 3  g -1),使用FESEM,BET进行评估,并具有通过各种电化学方法分析得到的优异的电化学行为。此外,组装的对称CBAC // CBAC器件在电流密度为0.2 A g -1时表现出240.8 F g -1的高比电容,并保持在65.6 F g -1的水平。在2.0 A g -1的高电流密度下。此外,该对称器件在400 W kg -1的比功率下可提供超过30 Wh kg -1的出色比能量最大值,并在超过5000次循环的长期中具有出色的循环稳定性。通过发光二极管测试该设备的操作。因此,基于CBAC的材料为开发用于能量存储设备应用的大规模,低成本材料铺平了道路。

更新日期:2021-03-01
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