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Testing topological phase transitions in Kitaev materials under in-plane magnetic fields: Application toα−RuCl3
Physical Review Research ( IF 3.5 ) Pub Date : 2021-02-24 , DOI: 10.1103/physrevresearch.3.013179
Jacob S. Gordon , Hae-Young Kee

Material realization of the non-Abelian Kitaev spin liquid phase—an example of Ising topological order (ITO)—has been the subject of intense research in recent years. The 4d honeycomb Mott insulator αRuCl3 has emerged as a leading candidate, as it enters a field-induced magnetically disordered state where a half-integer quantized thermal Hall conductivity κxy was reported. Further, a recent report of a sign change in the quantized κxy across a certain crystallographic direction is strong evidence for a topological phase transition between two ITOs with opposite Chern numbers. Although this is a fascinating result, independent verification remains elusive, and one may ask if there is a thermodynamic quantity sensitive to the phase transition. Here we propose that the magnetotropic coefficient k would serve such a purpose. We report a singular feature in k that indicates a topological phase transition across the b̂-axis where ITO is prohibited by a C2 symmetry. If the transition in αRuCl3 is indeed a direct transition between ITOs, or is a more broad realization of a topological phase transition, then this feature in k should be observable. Implications of C2 symmetry on other experimental quantities are also discussed.

中文翻译:

在平面磁场下测试Kitaev材料中的拓扑相变:在α-RuCl3中的应用

近年来,非阿贝尔Kitaev自旋液相的材料实现(伊辛拓扑顺序(ITO)的一个例子)一直是研究的主题。这4d 蜂窝莫特绝缘子 α-氯化钌3 进入场致磁无序状态,其中半整数量化的热霍尔电导率已成为领先的候选者 κXÿ已经报道。此外,最近的报告显示,量化后的符号变化κXÿ沿一定的晶体学方向的有力证据表明,两个Chern数相反的ITO之间存在拓扑相变。尽管这是一个令人着迷的结果,但是独立的验证仍然遥不可及,并且可能会问是否存在对相变敏感的热力学量。在这里,我们建议磁致系数ķ会达到这样的目的。我们在中报告了一个单一功能ķ 表示整个网络的拓扑相变 b̂禁止使用ITO的轴 C2对称。如果过渡在α-氯化钌3 确实是ITO之间的直接过渡,或者是拓扑相变的更广泛的实现,那么此功能 ķ应该是可观察的。的含义C2 还讨论了其他实验量的对称性。
更新日期:2021-02-24
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