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Electron–phonon coupling in superconducting 1T-PdTe 2
npj 2D Materials and Applications ( IF 9.1 ) Pub Date : 2021-02-23 , DOI: 10.1038/s41699-021-00204-5
Gloria Anemone , Pablo Casado Aguilar , Manuela Garnica , Fabian Calleja , Amjad Al Taleb , Chia-Nung Kuo , Chin Shan Lue , Antonio Politano , Amadeo L. Vázquez de Parga , Giorgio Benedek , Daniel Farías , Rodolfo Miranda

We have determined the electron–phonon interaction in type II Dirac semimetallic 1T-PdTe2 by means of helium atom scattering. While 1T-PdTe2 is isostructural with 1T-PtTe2, only the former is superconductor. The difference can be traced to the substantially larger value of the electron–phonon coupling in 1T-PdTe2, λ = 0.58, obtained from the Debye-Waller attenuation of the He specular peak. With this value and the surface Debye temperature, ΘD = 106.2 K, we have figured out the superconducting critical temperature, Tc = 1.83 K given by the BCS theory, which is in good agreement with Tc = (1.95 ± 0.03) K obtained with low-temperature scanning tunneling microscopy. The value of the effective mass related to ΘD indicates that the large electron–phonon coupling in 1T-PdTe2 is due to coupling, not only with the zone-center optical mode O2 at 9.2 meV, as proposed in a recent theoretical study, but also with the zone-boundary acoustic mode LA. Our results suggest that the topological states of a Dirac cone play a negligible role on the onset of superconductivity.



中文翻译:

1T-PdTe 2超导中的电子-声子耦合

我们已经通过氦原子散射确定了II型Dirac半金属1T-PdTe 2中的电子-声子相互作用。虽然1T-PdTe 2是同构与1T-PtTe 2,只有前者的超导体。可以追溯到1T-PdTe 2中电子-声子耦合的较大值,λ  = 0.58,这是从He镜面反射峰的Debye-Waller衰减获得的。随着该值和表面温度德拜,Θ d  = 106.2 K,我们已经想出超导临界温度,Ť Ç  =由BCS理论,这是在具有良好的协议给定的1.83ķ Ť Ç =(1.95±0.03)K是用低温扫描隧道显微镜得到的。有关Θ的有效质量的值d表示在1T-PdTe大电子-声子耦合2是由于耦合,不仅与该区域中心的光学模式ö 2在9.2兆电子伏,如在最近的理论研究中提出,也可以使用区域边界声学模式LA。我们的研究结果表明,狄拉克锥的拓扑状态在超导性的发生中起着微不足道的作用。

更新日期:2021-02-23
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