Moving from Fundamental Knowledge of Kinetics and Mechanisms on Surfaces to Prediction of Catalyst Performance in Reactors,ACS Catalysis

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Moving from Fundamental Knowledge of Kinetics and Mechanisms on Surfaces to Prediction of Catalyst Performance in Reactors
ACS Catalysis ( IF 11.3 ) Pub Date : 2021-02-23 , DOI: 10.1021/acscatal.0c05173
Christian Reece ₁ , Robert J. Madix ₂

Affiliation

Catalysis is defined by kinetics, but after over a century of catalyst development our kinetic and mechanistic knowledge governing real-world catalysis is still severely lacking. This Perspective considers how we can use the precise knowledge available from both theoretical and fundamental experimental techniques to understand and even predict catalytic performance under operational conditions. We describe advances that link fundamental and “real-world” measurements, crucial elements required to successfully recreate a reaction network, and avenues that appear to offer viable routes to success.

中文翻译：

从表面动力学和机理的基础知识到反应器中催化剂性能的预测

催化作用是由动力学定义的，但是经过一个多世纪的催化剂开发，我们仍然仍然缺乏控制现实世界催化作用的动力学和机理知识。本《观点》考虑了如何利用理论和基础实验技术中的精确知识来理解甚至预测运行条件下的催化性能。我们描述了将基本测量和“实际”测量，成功重建反应网络所需的关键要素以及似乎为成功提供可行途径的途径联系在一起的进步。

更新日期：2021-03-05

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