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Inverted planer perovskite solar cells fabricated by all vapor phase process
Japanese Journal of Applied Physics ( IF 1.5 ) Pub Date : 2021-02-10 , DOI: 10.35848/1347-4065/abdad3
Satoru Seto

A simple vapor-based fabrication process for perovskite solar cells is developed and applied to the fabrication of inverted planar CH3NH3PbI3 (MAPbI3) perovskite solar cells. In this process, PbI2 film is deposited by vacuum evaporation on the hole transport layer (HTL), followed by converting it into the MAPbI3 phase by annealing in methylammonium iodide (MAI) vapor. Using the converted MAPbI3 films, we fabricated inverted planar perovskite solar cells by vapor phase-based process with a device structure of glass/TCO/HTL/MAPbI3/C60/BCP/Ag, in which PEDOT:PSS and copper phthalocyanine (CuPc) were used as an HTL. A power conversion efficiency as high as 16.1% was obtained for the solar cell using CuPc as an HTL by a fully vapor-based process. Furthermore, we observed the improvement of the stability of the solar cells when using CuPc instead of PEDOT:PSS as an HTL.



中文翻译:

采用全气相法制造的倒置钙钛矿型太阳能电池

钙钛矿太阳能电池一个简单的基于气相制造工艺开发和应用,以反转平面CH的制造3 NH 3碘化铅3(MAPbI 3)的钙钛矿太阳能电池。在此过程中,通过真空蒸发将PbI 2膜沉积在空穴传输层(HTL)上,然后通过在甲基碘化碘(MAI)蒸气中退火将其转化为MAPbI 3相。使用转换后的MAPbI 3薄膜,我们通过基于气相的工艺制造了倒置平面钙钛矿太阳能电池,其器件结构为玻璃/ TCO / HTL / MAPbI 3 / C 60/ BCP / Ag,其中PEDOT:PSS和铜酞菁(CuPc)被用作HTL。使用CuPc作为HTL的太阳能电池通过完全基于蒸汽的工艺获得了高达16.1%的功率转换效率。此外,当使用CuPc代替PEDOT:PSS作为HTL时,我们观察到了太阳能电池稳定性的提高。

更新日期:2021-02-10
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