Surface Science ( IF 2.1 ) Pub Date : 2021-02-10 , DOI: 10.1016/j.susc.2021.121822 A.V. Matetskiy , N.V. Denisov , L.V. Bondarenko , A.Y. Tupchaya , D.V. Gruznev , A.N. Mihalyuk , A.V. Zotov , A.A. Saranin
Electronic and transport properties of the dense Pb/Si(100) reconstructions, 21-Pb with 1.5 ML (monolayer) of Pb and c(44)-Pb with 1.875 (15/8) ML of Pb, have been explored using angle-resolved photoelectron spectroscopy in conjunction with the DFT calculations and in situtransport and magnetotransport four-probe measurements at low temperatures. Both reconstructions are the low-dimensional materials with the advanced properties. In particular, the Pb/Si(100)21 shows up as a quasi-one-dimensional metallic phase with an extremely great spin splitting of the metallic surface-state band as revealed by the DFT calculations. The Pb/Si(100)c(44) has been found to demonstrate fingerprints of a superconductor with a critical temperature of 1.03 K. At low temperatures, the reconstructions display quantum phenomena relevant to their low-dimensional nature, e.g., metal-insulator transition for the Pb/Si(100)21 and magnetic-field-induced superconductor-insulator transition for the Pb/Si(100)c(44).
中文翻译:
Si(100)上Pb密集重构的电子和输运性质
致密Pb / Si(100)重建物的电子和输运性质,21-Pb与1.5 ML(单层)的Pb和c(44)-铅 使用角度分辨光电子能谱结合DFT计算以及低温下的原位传输和磁传输四探针测量,已经探索了1.875(15/8)ML的Pb 。两种重建都是具有先进特性的低维材料。特别是Pb / Si(100)2图1显示为准一维金属相,通过DFT计算可知,金属表面状态带具有极大的自旋分裂。铅/硅(100)c(44)已发现可显示临界温度为1.03 K的超导体的指纹。在低温下,该重建物显示与其低维性质有关的量子现象,例如Pb / Si(100)的金属-绝缘体跃迁21和Pb / Si(100)c(4)的磁场感应超导体-绝缘体跃迁4)。