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Rapid and precise measurements of radon in water using a pulsed ionization chamber
Limnology and Oceanography: Methods ( IF 2.1 ) Pub Date : 2021-02-01 , DOI: 10.1002/lom3.10419
Junhyeong Seo 1 , Guebuem Kim 1
Affiliation  

Radon‐in‐air monitor (RAD7, Durridge Co.) has been widely used to measure 222Rn in water samples. RAD7 measures 222Rn via 218Po+ (t1/2 = 3.1 min), which is electrically attracted to a silicon alpha detector. In this study, a new method was developed for measuring 222Rn in water samples by modifying a commercially available pulsed ionization chamber (PIC, FT‐Lab Co.). The PIC detects and amplifies the electric pulses generated by microspace charges produced by 222Rn decay. Two passive PICs (volume: 2 × 400 mL) were combined and modified to form an active system (named Rn‐SNU) that continuously circulates air (~ 1 L min−1). Rn‐SNU is approximately seven to nine times more efficient than RAD7 and does not necessitate a delay of ~ 15 min to reach radioactive equilibrium between 222Rn and 218Po+. However, RAD7 is more accurate in discriminating 222Rn daughters, 218Po+ and 214Po+. In this study, 222Rn was successfully measured in coastal seawater samples using Rn‐SNU connected to a grab bottle. Our results suggest that 222Rn measurements in water samples can be conducted more efficiently and rapidly with an Rn‐SNU than with other widely used instruments and methods.

中文翻译:

使用脉冲电离室快速准确地测量水中的don

in气监测仪(RAD7,Durridge公司)已被广泛用于测量水中的222 Rn。RAD7通过218 Po +t 1/2 = 3.1分钟)测量222 Rn ,该电被电吸引到硅α探测器。在这项研究中,通过修改市售的脉冲电离室(PIC,FT-Lab Co.),开发了一种用于测量水中样品中222 Rn的新方法。PIC检测并放大由222 Rn衰减产生的微空间电荷产生的电脉冲。合并并修改了两个无源PIC(体积:2×400 mL),形成了一个有源系统(命名为Rn-SNU),该系统使空气连续循环(〜1 L min -1)。Rn-SNU的效率大约是RAD7的7至9倍,并且无需延迟〜15分钟即可达到222 Rn和218 Po +之间的放射性平衡。但是,RAD7在区分222个Rn子代,218 Po +214 Po +时更为准确。在这项研究中,使用连接到抓瓶的Rn-SNU成功测量了沿海海水样品中的222 Rn。我们的结果表明,与其他广泛使用的仪器和方法相比,使用Rn-SNU可以更高效,更快速地进行222种水样品中的Rn测量。
更新日期:2021-02-01
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