Journal of Luminescence ( IF 3.3 ) Pub Date : 2021-01-30 , DOI: 10.1016/j.jlumin.2021.117924 Jacob S. Nyemann , Peter Balling , Eduardo G. Yukihara
The well-known thermoluminescent material LiF:Mg,Cu,P (MCP) was previously shown to emit significant optically stimulated luminescence (OSL). In this paper, we investigate the rate of OSL recombination processes in MCP, expressed as effective lifetimes, using time-correlated single photon counting, in this context often referred to as time-resolved pulsed OSL. The recombination luminescence fell into two categories: (i) a dominant fast decaying luminescence described by the two lifetimes and and (ii) a slowly decaying part with indeterminate decay profile at a comparatively low signal level (we denote this as “offset luminescence”). The fast recombination channels corresponding to and are responsible for of the total luminescence observed during test measurements. The luminescence associated with dominate the beginning of an experiment, but is depleted much quicker than the luminescence associated with . We show that all recombination channels show similar response to preheating of the sample, which suggests that they are associated with the same trapping centers.
中文翻译:
LiF:Mg,Cu,P的脉冲光激发发光的复合寿命
先前已显示众所周知的热致发光材料LiF:Mg,Cu,P(MCP)会发出明显的光学激发发光(OSL)。在本文中,我们使用时间相关的单光子计数来研究MCP中OSL重组过程的速率,将其表示为有效寿命,在这种情况下,通常将其称为时间分辨脉冲OSL。重组发光分为两类:(i)由两个寿命描述的主要快速衰变发光 和 (ii)在相对较低的信号电平下具有不确定衰减曲线的缓慢衰减部分(我们将其称为“偏移发光”)。对应的快速重组通道 和 负责 在测试测量中观察到的总发光量。与发光有关 在实验开始时占主导地位,但比与之相关的发光快得多 。我们显示,所有重组通道对样品的预热均显示相似的响应,这表明它们与相同的捕集中心相关。