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Effects of the spatial distribution of CO2 dilution on localised forced ignition of stoichiometric CH4 - CO2 - air mixtures
Combustion Theory and Modelling ( IF 1.9 ) Pub Date : 2021-01-27 , DOI: 10.1080/13647830.2021.1876926
Vassilios Stergios Papapostolou 1 , Charles Turquand d’Auzay 1, 2 , Nilanjan Chakraborty 1
Affiliation  

The localised forced ignition and subsequent flame propagation have been analysed for stoichiometric CH4CO2air mixtures with different spatial distributions and mean levels of CO2 dilution (i.e. mole fraction of CO2 in CH4/CO2 blend) for different flow conditions (e.g. quiescent laminar condition and different turbulence intensities) using three-dimensional Direct Numerical Simulations. The CH4+CO2 mixture is taken to represent biogas, as CH4 and CO2 are its two principal constituents. A two-step chemical mechanism, which has been demonstrated to capture the effects of CO2 dilution on the laminar burning velocity with sufficient accuracy, has been used for the purpose of a parametric analysis in terms of the mean value, standard deviation and integral length scale of the initial spatial Gaussian distributions of CO2 dilution in the unburned gas. An increase of mean CO2 dilution level was found to reduce the maximum values of temperature and the reaction rate magnitude of CH4. Moreover, an increase of mean CO2 dilution acts to reduce the probability of finding large reaction rate magnitudes of CH4, which also leads to a decreasing trend of burned gas volume CO2 irrespective of flow conditions. Furthermore, an increase in turbulence intensity acts to reduce the burned gas volume irrespective of mixture composition due to the enhancement of heat transfer from the hot gas kernel. However, the initial values of integral length scale and standard deviation of CO2 dilution variation (i.e. lψ and σψ) have been found not to have significant influences on the burned gas volume for the parameter range considered here. Although a small value of lψ promotes high rates of mixing of CO2 within the unburned gas, the overwhelming probability of finding CO2 dilution close to its mean value eclipses the effects of lψ and σψ even under laminar conditions, and this trend strengthens further under high turbulence intensities due to enhanced mixing.



中文翻译:

CO2稀释物的空间分布对化学计量CH4-CO2-空气混合物局部强制着火的影响。

分析了局部强制点火和随后的火焰传播的化学计量 CH4-CØ2个-空气 具有不同空间分布和平均水平的混合物 CØ2个 稀释度(即 CØ2个CH4/CØ2个使用三维直接数值模拟针对不同的流动条件(例如静态层流条件和不同的湍流强度)进行混合)。这CH4+CØ2个 混合物代表沼气,因为 CH4CØ2个是它的两个主要组成部分。两步化学机制已被证明可以捕获CØ2个 为了充分分析层流燃烧速度的稀释度,已将其用于初始空间高斯分布的均值,标准偏差和积分长度尺度用于参数分析。 CØ2个在未燃烧的气体中稀释。均值的增加CØ2个 发现稀释水平降低了温度的最大值和反应速率的幅度。 CH4。而且,均值的增加CØ2个 稀释作用降低了发现较大的反应速率幅度的可能性。 CH4,这也导致燃烧气体量减少的趋势 CØ2个不论流动条件如何。此外,湍流强度的增加起到减少燃烧气体体积的作用,而与混合物组成无关,这归因于来自热气体核的传热的增强。但是,积分长度刻度的初始值和标准偏差为CØ2个 稀释度变化(即 ψσψ对于此处考虑的参数范围,已发现)对燃烧的气体量没有显着影响。虽然价值不大ψ 促进高混合率 CØ2个 在未燃烧的气体中,发现的绝大多数可能性 CØ2个 接近其平均值的稀释会抵消 ψσψ 即使在层流条件下,由于增强了混合,这种趋势在高湍流强度下也会进一步增强。

更新日期:2021-01-27
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