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Plutonium and americium in the deep Black Sea bottom sediments
Journal of Environmental Radioactivity ( IF 1.9 ) Pub Date : 2021-01-24 , DOI: 10.1016/j.jenvrad.2021.106540
Vladislav Yu. Proskurnin , Nataliya N. Tereshchenko , Artem A. Paraskiv , Olga D. Chuzhikova-Proskurnina

The new data on 239+240Pu, 238Pu, 241Pu, 241Am vertical distribution in the deep western Black Sea sediments was analyzed. The sediment dating, obtained by means of 238Pu/239+240Pu activity ratio vertical distribution, suggested the upper 3 cm layer of sediments to be formed during 27 years after the Chernobyl accident and the deeper layers to be formed earlier in pre-Chernobyl time (before 1986). The whole data set on profiles of radionuclides studied was shown to reflect the history of their input into the basin and elimination of these radionuclides from the water column. Analysis of inventories of plutonium alpha-emitting nuclides ensured a more significant contribution of Chernobyl fallout into the present total 238Pu inventory than into 239+240Pu one. The 241Am inventory after-deposition enhancement due to 241Pu decay was estimated at 74% in pre-Chernobyl sediment layer and the general contribution of 241Pu support in the total 241Am inventory in situ enhancement was estimated at 49%.



中文翻译:

黑海深海沉积物中的and和a

分析了黑海西部西部沉积物中239 + 240 Pu,238 Pu,241 Pu,241 Am垂直分布的新数据。通过238 Pu / 239 + 240获得的沉积物测年Pu活度比的垂直分布,表明切尔诺贝利事故发生后27年内,上部3厘米的沉积层形成,切尔诺贝利事故发生前(1986年之前),较深层形成。显示了所研究放射性核素剖面的全部数据,以反映其向盆地输入以及从水柱中消除这些放射性核素的历史。对of发射核素的库存进行分析,确保切尔诺贝利尘埃落入当前238 pu的总存量比239 + 240 Pu的贡献更大。切尔诺贝利前沉积层中241 Pu衰减引起的241 Am沉积后沉积增强估计为74%,在总计241 Am的原位增强库存中,241 Pu支持估计为49%。

更新日期:2021-01-24
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