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Analysis of producing 238Pu as a byproduct in an MSFR
Annals of Nuclear Energy ( IF 1.9 ) Pub Date : 2021-01-20 , DOI: 10.1016/j.anucene.2020.108104
Ao Zhang , Chenggang Yu , Shaopeng Xia , Yong Cui , Chen Wu , Xiangzhou Cai , Jingen Chen

238Pu can be used as the heat source in radioisotope thermoelectric generators for deep space exploration, while it is currently in shortage because of the suspension of 238Pu production in the USA and Russia for many years. Two possible scenarios for the production of 238Pu as a byproduct in a molten salt fast reactor (MSFR) are assessed in this work. For the first scenario, the MSFR is started with low-enriched uranium (LEU), and neptunium is extracted from the fuel salt and then fed into the fertile salt of thorium for high-purity 238Pu production. For the second scenario, the ignition material for the MSFR is 233U, and highly purified 238Pu is produced by directly extracting plutonium from the fuel salt. The simulated results indicate that on average 15.48 kg 238Pu with the quality (ratio of 238Pu mass to total mass of Pu isotopes) larger than 98.6% can be produced per year during a 60-year operation for scenario I. In parallel, 8.31 kg 238Pu with the quality larger than 91.9% can be produced annually for scenario II. The 238Pu production has a small impact on the neutronic performance of the core for the two scenarios except that bred 238U is reduced by 922 kg for scenario I and by 261 kg for scenario II during the 60-year lifetime. The 238Pu production has a very tiny effect on the radiotoxicity of discharged nuclear fuel for scenario I, while it can reduce the total radiotoxicity of discharged nuclear fuel by three times for scenario II.



中文翻译:

在MSFR中产生副产物238 Pu的分析

238 Pu可以用作放射性同位素热电发生器中用于深空探测的热源,但由于美国和俄罗斯多年以来238 Pu生产的停产,目前短缺。在这项工作中,评估了在熔融盐快堆(MSFR)中生产副产物238 Pu的两种可能方案。对于第一种情况,MSFR首先从低浓铀(LEU)开始,然后从燃料盐中提取n,然后将其送入th的可育盐中,以高纯度生产238 Pu。对于第二种情况,MSFR的点火材料为233 U,高度净化的为238Pu是通过直接从燃油盐中提取p来生产的。模拟结果表明,对于方案I,在60年的运行期间,每年平均可以生产出15.48 kg 238 Pu,质量(238 Pu质量与Pu同位素总质量之比)大于98.6%。平行的是8.31方案II每年可生产质量大于91.9%的kg 238 Pu。在这两种情况下,238 Pu的产量对堆芯的中子学性能影响不大,不同的是,在60年的寿命中,情况I的繁殖的238 U减少了922 kg,情况II的减少了261 kg。在238Pu生产对方案I排放的核燃料的放射毒性影响很小,而对于方案II则可将排放的核燃料的总放射毒性降低三倍。

更新日期:2021-01-20
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