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Self-powered transparent photodetectors for broadband applications
Surfaces and Interfaces ( IF 5.7 ) Pub Date : 2021-01-10 , DOI: 10.1016/j.surfin.2021.100934
Thanh Tai Nguyen , Malkeshkumar Patel , Joondong Kim

Broadband transparent photodetectors are achieved through the formation of a metal oxide heterojunction. A high transmittance of 66.63% for visible light (400–800 nm) results from the wide energy bandgaps of TiO2 (3 eV) and NiO (3.86 eV). The metal-oxide heterojunction generates a photovoltaic effect due to the high open-circuit voltage (0.4 V), which spontaneously drives the NiO/TiO2 photodetector for self-powered operations. Therefore, the transparent NiO/TiO2 photodetector exhibits a self-operation mode with a fast response time (0.1 ms) while providing a high responsivity (0.43 A W−1) and detectivity (8.6 × 109 Jones) without any external bias. Extreme cycle testing (over 20,000 times) was performed to confirm the high stability of the transparent NiO/TiO2 photodetector. The proposed photovoltaic device can be an invisible power generator itself and be adopted for transparent optoelectronics, such as sensors, imaging, and memory applications with its self-operation mode.



中文翻译:

自供电的透明光电探测器,用于宽带应用

宽带透明光电探测器是通过形成金属氧化物异质结来实现的。TiO 2(3 eV)和NiO(3.86 eV)的宽能带隙使可见光(400-800 nm)的透射率达到66.63%。由于高的开路电压(0.4 V),金属氧化物异质结会产生光伏效应,从而自发地驱动NiO / TiO 2光电探测器进行自供电操作。因此,透明NiO / TiO 2光电探测器表现出具有快速响应时间(0.1 ms)的自操作模式,同时提供高响应度(0.43 AW -1)和检测率(8.6×10 9)琼斯),没有任何外部偏见。进行了极端循环测试(超过20,000次)以确认透明NiO / TiO 2光电探测器的高稳定性。所提出的光伏装置本身可以是不可见的发电机,并且可以通过其自操作模式用于透明的光电器件,例如传感器,成像和存储应用。

更新日期:2021-01-21
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