Zeolite membrane reactors: from preparation to application in heterogeneous catalytic reactions,Reaction Chemistry & Engineering

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Zeolite membrane reactors: from preparation to application in heterogeneous catalytic reactions
Reaction Chemistry & Engineering ( IF 3.4 ) Pub Date : 2020-12-11 , DOI: 10.1039/d0re00388c
I. G. Wenten _{1,

2,

3,

4,

5} , K. Khoiruddin _{1,

2,

3,

4,

5} , R. R. Mukti _{3,

4,

5,

6,

7} , W. Rahmah _{1,

2,

3,

4,

5} , Z. Wang _{8,

9,

10} , S. Kawi _{8,

9,

10}

Affiliation

Chemical reactions are some of the most crucial processes in industry for creating various important products. Coupling a chemical reaction with membrane separation, also known as a membrane reactor (MR), has been demonstrated in numerous studies, and it has been shown that this strategy can successfully meet the goal of process intensification. Among the membrane materials used, crystalline zeolites display various advantages due to their tailorable pore sizes and physicochemical properties. The traditional applications of zeolite membranes in reactors can be advanced, as zeolites may catalytically convert molecules in a selective manner during equilibrium-controlled reactions. Zeolite membrane reactors (ZMRs) can withstand harsh conditions, allowing their operation over wide ranges of temperature and pressure. This paper reviews various aspects of ZMRs comprehensively, including separation performance, catalytic activity, preparation methods, and potential applications in various reactions. In addition, the final part of this paper also discusses a comparative study of zeolites with metal–organic frameworks to anticipate the future of ZMRs.

中文翻译：

沸石膜反应器：从制备到在多相催化反应中的应用

化学反应是工业上生产各种重要产品的一些最关键过程。在众多研究中已证明，将化学反应与膜分离（也称为膜反应器（MR））相结合，已表明该策略可以成功满足过程强化的目标。在所用的膜材料中，结晶沸石由于其可调节的孔径和理化性质而显示出各种优点。可以改进在反应器中沸石膜的传统应用，因为在平衡控制的反应中，沸石可以选择性地催化转化分子。沸石膜反应器（ZMRs）可以承受苛刻的条件，因此可以在很宽的温度和压力范围内运行。本文全面综述了ZMR的各个方面，包括分离性能，催化活性，制备方法以及在各种反应中的潜在应用。此外，本文的最后部分还讨论了具有金属有机骨架的沸石的比较研究，以预测ZMR的未来。

更新日期：2021-01-04

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