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Isotropic Pauli-limited superconductivity in the infinite-layer nickelate Nd0.775Sr0.225NiO2
Nature Physics ( IF 17.6 ) Pub Date : 2021-01-04 , DOI: 10.1038/s41567-020-01128-5
Bai Yang Wang , Danfeng Li , Berit H. Goodge , Kyuho Lee , Motoki Osada , Shannon P. Harvey , Lena F. Kourkoutis , Malcolm R. Beasley , Harold Y. Hwang

The recent observation of superconductivity in thin-film infinite-layer nickelates1,2,3 offers a different angle from which to investigate superconductivity in layered oxides4. A wide range of candidate models have been proposed5,6,7,8,9,10, which emphasize single- or multi-orbital electronic structure, Kondo or Hund’s coupling and analogies to cuprates. Further experimental characterization of the superconducting state is needed to develop a full understanding of the nickelates. Here we use magnetotransport measurements to probe the superconducting anisotropy in Nd0.775Sr0.225NiO2. We find that the upper critical field is surprisingly isotropic at low temperatures despite the layered crystal structure. In a magnetic field, the superconductivity is strongly Pauli-limited, such that the paramagnetic effect dominates over orbital de-pairing. Underlying this isotropic response is a substantial anisotropy in the superconducting coherence length, which is at least four times longer in-plane than out-of-plane. A prominent low-temperature upturn in the upper critical field indicates the presence of an unconventional ground state.



中文翻译:

无限层镍酸盐 Nd0.775Sr0.225NiO2 中的各向同性泡利限制超导性

最近对薄膜无限层镍酸盐1,2,3中超导性的观察为研究层状氧化物4中的超导性提供了不同的角度。已经提出了广泛的候选模型5,6,7,8,9,10,它们强调单轨道或多轨道电子结构、Kondo 或 Hund 的耦合以及与铜酸盐的类比。需要对超导状态进行进一步的实验表征,以全面了解镍酸盐。在这里,我们使用磁输运测量来探测 Nd 0.775 Sr 0.225 NiO 2中的超导各向异性. 我们发现,尽管存在层状晶体结构,但上临界场在低温下却令人惊讶地各向同性。在磁场中,超导性受到强烈的泡利限制,因此顺磁效应在轨道去配对中占主导地位。这种各向同性响应的基础是超导相干长度的显着各向异性,其平面内至少是平面外的四倍。上临界场中显着的低温上升表明存在非常规基态。

更新日期:2021-01-04
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