Nano Polymorphism‐Enabled Redox Electrodes for Rechargeable Batteries,Advanced Materials

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Nano Polymorphism‐Enabled Redox Electrodes for Rechargeable Batteries
Advanced Materials ( IF 27.4 ) Pub Date : 2020-12-31 , DOI: 10.1002/adma.202004920
Jun Mei _{1,

2} , Jinkai Wang _{3,

4} , Huimin Gu ₃ , Yaping Du ₅ , Hongkang Wang ₄ , Yusuke Yamauchi _{6,

7} , Ting Liao _{2,

8} , Ziqi Sun _{1,

2} , Zongyou Yin ₃

Affiliation

School of Chemistry and Physics Queensland University of Technology Brisbane QLD 4000 Australia
Centre for Materials Science Queensland University of Technology Brisbane QLD 4000 Australia
Research School of Chemistry Australian National University Canberra ACT 2601 Australia
State Key Lab of Electrical Insulation and Power Equipment Center of Nanomaterials for Renewable Energy (CNRE) School of Electrical Engineering Xi'an Jiaotong University Xi'an 710049 China
School of Materials Science and Engineering & National Institute for Advanced Materials Energy Materials Chemistry Tianjin Key Lab for Rare Earth Materials and Applications Centre for Rare Earth and Inorganic Functional Materials Nankai University Tianjin 300350 China
School of Chemical Engineering and Australian Institute for Bioengineering and Nanotechnology The University of Queensland St Lucia QLD 4072 Australia
JST‐ERATO Yamauchi's Materials Space‐Tectonics Project 4‐1‐8 Honcho Kawaguchi Saitama 332‐0012 Japan
School of Mechanical Medical & Process Engineering Queensland University of Technology Brisbane QLD 4000 Australia

Nano polymorphism (NPM), as an emerging research area in the field of energy storage, and rechargeable batteries, have attracted much attention recently. In this review, the recent progress on the composition and formation of polymorphs, and the evolution processes of different redox electrodes in rechargeable metal‐ion, metal–air, and metal–sulfur batteries are highlighted. First, NPM and its significance for rechargeable batteries are discussed. Subsequently, the current NPM modulation strategies of different types of representative electrodes for their corresponding rechargeable battery applications are summarized. The goal is to demonstrate how NPM could tune the intrinsic material properties, and hence, improve their electrochemical activities for each battery type. It is expected that the analysis of polymorphism and electrochemical properties of materials could help identify some “processing–structure–properties” relationships for material design and performance enhancement. Lastly, the current research challenges and potential research directions are discussed to offer guidance and perspectives for future research on NPM engineering.

中文翻译：

可充电电池的纳米多态性氧化还原电极

纳米多态性（NPM）作为储能和可充电电池领域的新兴研究领域，最近引起了广泛关注。在这篇综述中，重点介绍了多晶型物的组成和形成方面的最新进展，以及可再充电金属离子，金属空气和金属硫电池中不同氧化还原电极的演变过程。首先，讨论了NPM及其对可充电电池的意义。随后，总结了针对其相应的可再充电电池应用的不同类型的代表性电极的当前NPM调制策略。目的是证明NPM如何调节固有的材料性能，从而改善每种电池类型的电化学活性。可以预期，对材料的多态性和电化学性能进行分析可以帮助确定一些“加工-结构-性能”关系，以进行材料设计和性能提升。最后，讨论了当前的研究挑战和潜在的研究方向，以为NPM工程的未来研究提供指导和观点。

更新日期：2021-02-22

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