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Determination of the long-lived 10Be in construction materials of nuclear power plants using photoactivation method
Journal of Environmental Radioactivity ( IF 1.9 ) Pub Date : 2020-12-13 , DOI: 10.1016/j.jenvrad.2020.106509
V.A. Zheltonozhsky , D.E. Myznikov , V.I. Slisenko , M.V. Zheltonozhskaya , A.P. Chernyaev

The problem of handling nuclear power plant irradiated structural materials holds one of the central places in the nuclear power industry. High toxic 10Be with a half-life of T1/2 = 1.6 × 106 years is discovered in NPP structural materials after reactor operating. 10Be decays through only electrons' emission. Pure beta emitters are extremely difficult to determine in irradiated structural materials and radioactive waste. We proposed a photoactivation approach for determining the 10Be activity in NPP samples. The proposed method involves determining 9Be and 10B concentrations and subsequent recalculation of 10Be activity formed in 9Be(n, γ)10Be and 10B(n, p)10Be reactions. The amount of 9Be and 10B is determined by samples' photoactivation using an electron accelerator and 9Be(γ, 2n)7Be-, 10B(γ, p2n)7Be-reactions. These reactions' experimental yields were measured for 20, 40, and 55 MeV boundary energies of the bremsstrahlung beam. The proposed technique was tested on samples of ChNPP 2nd unit irradiated structural materials. The technique's calculated error is about 15–20%; the sensitivity is 1 Bq × g−1.



中文翻译:

光活化法测定核电站建筑材料中长寿命10 Be

处理核电站辐射的结构材料的问题是核电工业的中心位置之一。反应堆运行后,在NPP结构材料中发现了半衰期为T 1/2  = 1.6×10 6年的高毒10 Be 。10 Be仅通过电子的发射而衰减。在辐射的结构材料和放射性废物中,很难确定纯β发射体。我们提出了一种光活化方法来确定NPP样品中的10 Be活性。拟议的方法涉及确定9 Be和10 B的浓度,然后重新计算10 Be中形成的10 Be活性。9 Be(n,γ)10 Be和10 B(np10 Be反应。量9 Be和10 B由样本的光活化使用电子加速器和确定9为(γ,2 Ñ7 BE-,10 B(γ,p 2 Ñ7 BE-反应。测量了ms致辐射束的20、40和55 MeV边界能的这些反应的实验产率。所提出的技术是关于ChNPP跟2的样品测试第二单元辐照的结构材料。该技术的计算误差约为15–20%。灵敏度为1 Bq×g -1

更新日期:2020-12-14
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