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Magnetically separable highly efficient full-spectrum light-driven WO2.72/Fe3O4 nanocomposites for photocatalytic reduction of carcinogenic chromium (VI) and organic dye degradation
Journal of the Taiwan Institute of Chemical Engineers ( IF 5.5 ) Pub Date : 2020-12-10 , DOI: 10.1016/j.jtice.2020.12.006
Kebena Gebeyehu Motora , Chang-Mou Wu

In this study, magnetically separable, highly efficient full-spectrum light active WO2.72/Fe3O4 nanocomposites were synthesized by a solvothermal method and well characterized. The photocatalytic property of WO2.72/Fe3O4 nanocomposite toward photodegradation of methylene blue (MB), methyl orange (MO), and rhodamine B (Rh B) dyes under solar and photoreduction of Cr(VI) under ultraviolet (UV), visible, and solar light were studied. The WO2.72/Fe3O4 nanocomposite exhibited excellent photocatalytic activity for the photodegradation of MO, MB, and Rh B dyes under solar light and photoreduction of Cr(VI) under visible, UV, and solar light. The WO-FO-0.5 nanocomposite exhibited 2.9, 1.6, and 2.0 times the photocatalytic activity of Fe3O4 for Cr(VI) photoreduction under solar, visible, and UV and 20, 29.2, and 16 times that of Fe3O4, for Rh B, MB, and MO under solar light. It doesn't show only universal applicability for photocatalysis of different organic and inorganic pollutants but, also outstanding stability and easy separability. The nanocomposite also exhibited higher photocatalytic activity than that reported for photoreduction Cr(VI) under solar light. It is also convenient for large-scale applications due to its low cost, eco-friendliness, and easy preparation. Therefore, it is a promising candidate for environmental remediation under full-spectrum solar light.



中文翻译:

磁分离高效全光谱光驱动WO 2.72 / Fe 3 O 4纳米复合材料,用于光催化还原致癌铬(VI)和有机染料降解

在这项研究中,通过溶剂热法合成了磁可分离,高效的全光谱光活性WO 2.72 / Fe 3 O 4纳米复合材料,并对其进行了很好的表征。WO 2.72 / Fe 3 O 4纳米复合材料对亚甲基蓝(MB),甲基橙(MO)和若丹明B(Rh B)染料在太阳光下光降解Cr(VI)和在紫外线(UV)下光还原的光催化性能,可见光,并研究了太阳光。WO 2.72 / Fe 3 O 4纳米复合材料对MO,MB和Rh B染料在太阳光下的光降解以及Cr(VI)在可见光,UV和太阳光下的光还原表现出优异的光催化活性。在WO-FO-0.5纳米复合材料显示出2.9,1.6,和Fe的2.0倍的光催化活性3 ö 4为铬(VI)下的太阳能,可见光还原,和UV和20,29.2,和16倍的Fe 3 ö 4 ,在太阳光下用于Rh B,MB和MO。它不仅显示出对各种有机和无机污染物的光催化作用的普遍适用性,而且还具有出色的稳定性和易分离性。该纳米复合材料还显示出比报道的在太阳光下光还原Cr(VI)更高的光催化活性。由于其低成本,生态友好和易于制备,因此也便于大规模应用。因此,它是在全光谱太阳光下进行环境修复的有希望的候选者。

更新日期:2021-01-29
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