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Polymer fused GOFe: Light-driven oxygen donor and antiseptics
Journal of Photochemistry and Photobiology A: Chemistry ( IF 4.1 ) Pub Date : 2020-12-07 , DOI: 10.1016/j.jphotochem.2020.113075
Wei-Yu Mu , Wei Wang , Qiu-Yun Chen , Ling-Ling Qu

Phytopathogenic bacteria have been a prominent problem for the growth of plant and agricultural development. Iron-based oxygen generators will be environmental friendly materials for the treatment of phytopathogenic bacteria in hypoxia environment. To develop environmental friendly materials for bacterial treatment, a polymer fused iron(III) nano-complex (PPaba-FeEu@GO) was constructed. The PPaba-FeEu@GO was synthesized by polymerization of 4-aminobenzoic acid Fe(III) complex on the surface of 0.1 % Eu(III)-doped GO. This nano metal complex (PPaba-FeEu@GO) shows enhanced electron mobility and hole diffusion distance, hence it converts water into oxygen under LED light irradiation without adscititious cocatalyst. Moreover, PPaba-FeEu@GO can convert near-infrared light into heat. The photothermal conversion efficiency was calculated as 40.6 %. Therefore, PPaba-FeEu@GO is a light driven oxygen generator and bacterial inhibitor. Our results demonstrate that polymer fused metal-EuGO system will be kinds of reusable materials for bacterial treatment.



中文翻译:

聚合物熔合GOFe:光驱供氧体和防腐剂

植物病原菌一直是植物生长和农业发展的突出问题。铁基氧气发生器将是低氧环境中治疗植物致病细菌的环保材料。为了开发用于细菌处理的环保材料,构建了聚合物熔铁(III)纳米复合物(PPaba-FeEu @ GO)。PPaba-FeEu @ GO是通过在0.1%Eu(III)掺杂的GO表面上聚合4-氨基苯甲酸Fe(III)配合物而合成的。这种纳米金属配合物(PPaba-FeEu @ GO)表现出增强的电子迁移率和空穴扩散距离,因此在LED光照射下将水转化为氧气而没有助催化剂。此外,PPaba-FeEu @ GO可以将近红外光转换为热量。计算出光热转化效率为40.6%。因此,PPaba-FeEu @ GO是一种光驱氧气发生器和细菌抑制剂。我们的结果表明,聚合物熔融金属-EuGO系统将是可重复使用的细菌处理材料。

更新日期:2021-01-11
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