Abstract

We predict the characteristics of hyperfine interactions (hfi) for a number of electron-nuclear spin systems NV-¹³C in diamonds grown by seeding approach from the specific isotopic aza-adamantane or methyl-aza-adamantane molecules differing in ¹³C position in the precursor as well as in the orientation of the NV center in the post-obtained diamond. For the purpose we have used the spatial and hfi data simulated previously for the cluster C₅₁₀[NV]^–H₂₅₂. The data obtained can be used to identify (and correlate with the precursor used) the specific NV-¹³C spin system by measuring the hfi-induced splitting in optically detected magnetic resonance spectra being characteristic for the NV-¹³C system.

中文翻译：

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同位素氮杂金刚烷和甲基氮杂金刚烷的晶种方法形成的金刚石纳米晶体中的量子寄存器NV-13С的超精细特征

摘要

我们通过从不同的同位素氮杂金刚烷或甲基氮杂金刚烷分子在¹³ C位置不同的特定播种方法来预测钻石中许多电子核自旋系统NV- ¹³ C的超精细相互作用（hfi）的特征。前钻石以及后获得钻石中NV中心的方向。为此，我们使用了先前为群集C ₅₁₀ [NV] ^– H ₂₅₂模拟的空间和hfi数据。获得的数据可用于通过测量hfi来识别特定的NV- ¹³ C自旋系统（并与使用的前体相关）在光学检测到的磁共振光谱中引起的分裂是NV- ¹³ C系统的特征。