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Enhanced energy storage properties of ZrO2-doped (Na0.5Bi0.5)0.4Sr0.6TiO3 Pb-free relaxor ferroelectric ceramics
Ceramics International ( IF 5.1 ) Pub Date : 2020-12-01 , DOI: 10.1016/j.ceramint.2020.11.222
Biao Guo , Leiyang Zhang , Jia Dong , Yang Li , Fukang Chen , Qiao Ai , Quan Li , Zhanbing He , Yan Yan , Dawei Wang

Abstract (Na0.5Bi0.5)0.4Sr0.6Ti1-xZrxO3 relaxor ferroelectric ceramic were prepared by a traditional ceramic preparation process introducing Zr4+ at the B-site. It was observed that introducing an appropriate amount of Zr4+ ions into the NBST matrix can improve the energy storage efficiency. (Na0.5Bi0.5)0.4Sr0.6Ti0.5Zr0.5O3 shows excellent energy storage density up to 2.83 J/cm3, and excellent efficiency (83.90 %) at 220 kV/cm. A single layer ceramic capacitor (SLCC) was also prepared by the tape casting technique for multilayer ceramic capacitors (MLCCs) to further enhance the energy storage performance. The recoverable energy storage capacity is increased to 4.52 J/cm3 and the efficiency is 70.02 % at 460 kV/cm. Moreover, it still has a relatively stable energy storage performance after 105 cycles of charge and discharge. This sample has exhibited outstanding energy storage performance, fatigue resistance, and charge/discharge performance and has great potential value in practical applications.

中文翻译:

ZrO2掺杂(Na0.5Bi0.5)0.4Sr0.6TiO3无铅弛豫铁电陶瓷增强储能性能

摘要 (N​​a0.5Bi0.5)0.4Sr0.6Ti1-xZrxO3弛豫铁电陶瓷采用传统陶瓷制备工艺,在B位引入Zr4+。观察到在 NBST 基质中引入适量的 Zr4+ 离子可以提高储能效率。(Na0.5Bi0.5)0.4Sr0.6Ti0.5Zr0.5O3 显示出高达 2.83 J/cm3 的出色储能密度,以及在 220 kV/cm 下的出色效率 (83.90 %)。还通过用于多层陶瓷电容器(MLCC)的流延技术制备了单层陶瓷电容器(SLCC),以进一步提高储能性能。可恢复的储能容量增加到 4.52 J/cm3,在 460 kV/cm 下的效率为 70.02%。而且,经过105次充放电循环后,仍具有相对稳定的储能性能。
更新日期:2020-12-01
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