A nanoporous all-solid-state MOF-laden polymer electrolyte that is simply mediated by an electronic effect shows remarkably high lithium electrodeposition stability of hundreds of charge–discharge cycles and over 1500 operating hours, while maintaining a very small voltage polarization. This result is a significant improvement relative to conventional PEO and, when used in an all-solid-state battery (ASSB), this electrolyte enabled enhanced cycle life. This new all-solid-state electrolyte shows a promising rational design for the emerging microporous polymeric materials as novel SPEs in ASSBs.

中文翻译：

---

一种功能化的负载金属有机骨架的纳米多孔聚合物电解质，可实现极其稳定的锂电沉积

简单地通过电子效应介导的纳米多孔全固态MOF聚合物电解质在数百次充放电循环和超过1500个工作小时的过程中显示出极高的锂电沉积稳定性，同时保持了非常小的电压极化。与传统的PEO相比，此结果是一项显着的改进，当用于全固态电池（ASSB）中时，这种电解质可以延长循环寿命。这种新型的全固态电解质为新兴的微孔聚合物材料（如ASSB中的新型SPE）显示了一种有希望的合理设计。