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The effect of a ruthenium precursor on the low-temperature ammonia synthesis activity over Ru/CeO2
Dalton Transactions ( IF 4 ) Pub Date : 2020-11-25 , DOI: 10.1039/d0dt01974g
Yuichi Manaka 1, 2, 3, 4, 5 , Yuki Nagata 1, 2, 3, 4, 6 , Keisuke Kobayashi 1, 2, 3, 4 , Daisuke Kobayashi 4, 6, 7, 8 , Tetsuya Nanba 1, 2, 3, 4
Affiliation  

Catalysts supported on CeO2 were prepared using various Ru precursors. The H2-TPR profile of the catalyst was obtained beginning at −70 °C for the first time, and a previously unreported reduction peak was observed at approximately 50 °C. The lower peak temperature was associated with a higher ammonia synthesis activity.

中文翻译:

Ru / CeO2上钌前驱物对低温氨合成活性的影响

使用各种Ru前体制备负载在CeO 2上的催化剂。首次从-70°C开始获得催化剂的H 2 -TPR曲线,并在约50°C观察到先前未报告的还原峰。较低的峰值温度与较高的氨合成活性有关。
更新日期:2020-11-25
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