Mechanism and origins of regioselectivities of Rh-catalyzed alkenylation of allylbenzenes,Dalton Transactions

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Mechanism and origins of regioselectivities of Rh-catalyzed alkenylation of allylbenzenes
Dalton Transactions ( IF 3.5 ) Pub Date : 2020-11-04 , DOI: 10.1039/d0dt03704d
Tian-Qi Li _{1,

2,

3,

4} , Jing-Yi Tan _{1,

2,

3,

4} , Wei Deng _{1,

2,

3,

4} , Zheng-Yang Xu _{1,

2,

3,

4}

Affiliation

Rhodium-catalyzed alkenylation of allylbenzene derivatives via C–C bond activation provides an unprecedented access to alkenylation products with remarkable regioselectivities. Using DFT calculations, we elucidate the reaction mechanism and the origins of the regioselectivity.

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