Covalent Organic Frameworks in Catalytic Organic Synthesis,Advanced Synthesis & Catalysis

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Covalent Organic Frameworks in Catalytic Organic Synthesis
Advanced Synthesis & Catalysis ( IF 4.4 ) Pub Date : 2020-11-17 , DOI: 10.1002/adsc.202001086
Hai‐Yang Cheng ₁ , Tao Wang ₁

Affiliation

Covalent organic frameworks (COFs), which are built upon dynamic covalent chemistry (DCC) with various organic building blocks, possess predesignable, highly ordered and crystalline porous structures. These features endow COFs with great potential in the development of function‐tailored materials, particularly in catalytic organic synthesis. Start from selective oxidation reactions early introduced by Ferdi, Thomas and their co‐workers, and then Wang and co‐workers performed Suzuki‐Miyaura reaction through integrating palladium into COFs, increasing numbers of works were established to explore their potentials in the 4.5catalysis of organic reactions. As heterogeneous organic catalysts, COFs bring benefits and solve problems, but also create new obstacles. Hence, we would like to establish a comprehensive system to review some pioneering works in this area. This will help us get a better view so that we can discuss the key and challenging issues we are currently confronted with.

中文翻译：

催化有机合成中的共价有机骨架

共价有机骨架（COF）建立在具有各种有机构件的动态共价化学（DCC）之上，具有可预先设计，高度有序和结晶的多孔结构。这些功能使COF在功能定制材料的开发中具有巨大潜力，尤其是在催化有机合成中。从Ferdi，Thomas及其同事早期引入的选择性氧化反应开始，然后Wang和同事通过将钯整合到COF中进行铃木-宫浦反应，建立了越来越多的工作以探索它们在4.5催化中的潜力。有机反应。作为非均质有机催化剂，COF既带来了好处并解决了问题，也带来了新的障碍。因此，我们想建立一个全面的系统来审查该领域的一些开拓性工作。这将有助于我们更好地了解自己，以便我们可以讨论当前面临的关键和挑战性问题。

更新日期：2021-01-05

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