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Soot maturity studies in methane-air diffusion flames at elevated pressures using laser-induced incandescence
Proceedings of the Combustion Institute ( IF 5.3 ) Pub Date : 2020-11-17 , DOI: 10.1016/j.proci.2020.07.127
Manu Mannazhi , Sandra Török , Jinlong Gao , Per-Erik Bengtsson

Two-dimensional laser-induced incandescence (LII) measurements were used for quantitative soot volume fraction (fv) measurements in methane-air diffusion flames at pressures ranging from 0.1 to 0.5 MPa. Additionally, laser-induced fluorescence (LIF) was used for visualization of polycyclic aromatic hydrocarbons (PAHs) considered as important soot precursors. A heat and mass transfer-based LII model was used for the analysis of experimental LII fluence curves to evaluate soot absorption functions, E(m), at various spatial positions in the flames. Based on previous work, variations in the evaluated E(m) was assumed to be related to soot maturity. Generally, the most mature soot was found at the spatial position of maximum fv along the central axis and at the flame edges. Also, the soot maturity at the position of maximum fv at each pressure was found to increase from the flame at 0.1 MPa to 0.5 MPa. A critical examination of the assumptions and uncertainties in the E(m) analysis was made. The present study emphasizes the limitation of assigning soot a constant E(m) in the overall flame for temperature and soot concentration evaluation using the optical methods spectral soot emission (SSE) and line-of-sight attenuation (LOSA), which are commonly used non-intrusive optical diagnostic techniques in sooting high-pressure flames. The study also demonstrates the critical choice of fluence in quantitative imaging LII measurements of fv when the E(m) of soot spans over large range of values.



中文翻译:

使用激光诱导的白炽灯研究高压下甲烷-空气扩散火焰中的烟尘成熟度

二维激光诱导白炽度(LII)测量用于定量烟灰体积分数(Fv)在压力为0.1至0.5 MPa的甲烷-空气扩散火焰中进行测量。此外,激光诱导荧光(LIF)用于可视化为重要烟灰前体的多环芳烃(PAH)。基于传热和传质的LII模型用于分析实验性LII能量密度曲线,以评估烟灰吸收功能,Ë在火焰中的各个空间位置。根据以前的工作,评估Ë被认为与烟灰的成熟有关。通常,最成熟的烟灰位于最大烟灰的空间位置。Fv沿中心轴和火焰边缘。另外,最大位置的烟灰成熟度Fv发现在每个压力下,火焰在0.1MPa下的最大压力增加到0.5MPa。批判性地考察了假设中的假设和不确定性Ë分析。本研究强调了为烟灰分配常数的局限性Ë使用光谱方法的光谱烟尘发射(SSE)和视线衰减(LOSA)评估整体火焰中的温度和烟灰浓度,这是在高压烟灰中常用的非侵入式光学诊断技术。该研究还证明了定量成像LII测量中注量的关键选择Fv 当。。。的时候 Ë 烟尘跨度很大。

更新日期:2020-11-17
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