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Construction of a low-temperature, highly sensitive H2S sensor based on surfaces and interfaces reaction triggered by Au-doped hierarchical structured composites
Chemical Physics Letters ( IF 2.8 ) Pub Date : 2020-11-16 , DOI: 10.1016/j.cplett.2020.138188
Shaohui Zhang , Zeng Liu , Long Zhang , Jiafan Chen , Quan Zhou , Haifeng Zhang , Lifan Nie , Zhaobo Dong , Zi'ang Zhang , Zugang Wang , Gebo Pan

A low-temperature, highly sensitive H2S sensor based on Au-doped ZnO/Zn2SnO4 (AZZ) hierarchical structured composites was fabricated by using a screen printing craft. With the introduction of Au, the response of the AZZ-based sensor to H2S is improved from 2.1 to 15.92 at 150 °C for a [Au]/[Zn] molar ratio of 0.1%. Moreover, the as-prepared sensor has better selectivity to H2S. It is worth mentioning that the sensor shows a commendable ultra-fast recovery time (2 s). Importantly, the unique AZZ hierarchical structure is conducive to chemical adsorption, surfaces and interfaces reactions, gas diffusion and transmission, thereby enhancing the sensing performance.



中文翻译:

基于金掺杂的分层结构复合材料引发的表面和界面反应构建低温,高灵敏度的H 2 S传感器

通过使用丝网印刷工艺,制造了一种基于Au掺杂的ZnO / Zn 2 SnO 4(AZZ)分层结构化复合材料的低温,高灵敏度H 2 S传感器。随着Au的引入,对于[Au] / [Zn]摩尔比为0.1%的情况,基于AZZ的传感器对H 2 S的响应在150°C时从2.1提高到15.92。而且,所制备的传感器对H 2 S具有更好的选择性。值得一提的是,该传感器显示出值得称赞的超快恢复时间(2 s)。重要的是,独特的AZZ分层结构有利于化学吸附,表面和界面反应,气体扩散和传输,从而增强了传感性能。

更新日期:2020-11-16
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