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Intensification of Ozone Generation and Degradation of Azo Dye in Non-Thermal Hybrid Corona-DBD Plasma Micro-Reactor
Chemical Engineering and Processing: Process Intensification ( IF 3.8 ) Pub Date : 2020-11-11 , DOI: 10.1016/j.cep.2020.108205
Ainy Hafeez , Fahed Javed , Tahir Fazal , Nasir Shezad , Um-e-Salma Amjad , Muhammad Saif ur Rehman , Fahad Rehman

A novel corona-dielectric barrier discharge hybrid non-thermal plasma micro-reactor was investigated for ozone generation and pollutant degradation. It was hypothesized that creating a submicron channel inside the micro-reactor would increase ozone generation efficiency. Therefore, the plasma micro-reactor was packed with dielectric glass beads. The plasma micro-reactor operating conditions were investigated for ozone formation. The efficiency of the empty channel plasma reactor was compared with the packed-bed plasma reactor which was 24% higher than the former at optimized conditions-5 kV peak voltage, 36 mA peak current, 26.02 kHz frequency, 1 Lmin-1 air flow rate, and 4 cm electrode length. The performance of the reactor was evaluated for the degradation of Reactive black-5. The plasma micro-reactor operating conditions and the dye operational parameters- pH of the solution, initial dye concentration, and volume of solution were also investigated to see the efficiency of reactive black-5 removal in the plasma reactor. The dye degradation efficiency increased by 50% in the packed-bed plasma micro-reactor as compared to the empty channel reactor. In the empty channel reactor, 98% reactive-black-5 was removed with 87% COD reduction in 16 minutes, and in the packed-bed reactor, 98.3% was removed with 89% COD reduction in 8 min of the plasma treatment.



中文翻译:

非热电晕-DBD等离子体微反应器中臭氧产生的加剧和偶氮染料的降解

研究了一种新型的电晕-电介质阻挡放电混合非热等离子体微反应器,用于产生臭氧和降解污染物。假设在微反应器内部建立亚微米通道将增加臭氧的产生效率。因此,等离子微反应器填充有介电玻璃珠。研究了等离子体微反应器的操作条件以了解臭氧的形成。将空通道等离子体反应器的效率与填充床等离子体反应器进行了比较,后者在优化条件下比前者高了24%。5kV峰值电压,36 mA峰值电流,26.02 kHz频率,1 Lmin -1空气流速和4 cm电极长度。评价反应器性能以反应性黑5的降解。还研究了等离子体微反应器的操作条件和染料的操作参数-溶液的pH值,初始染料浓度和溶液的体积,以了解在等离子体反应器中去除活性黑5的效率。与空通道反应器相比,填充床等离子体微反应器的染料降解效率提高了50%。在空通道反应器中,在16分钟内以98%的COD降低去除了98%的活性黑5,而在填充床反应器中,在等离子处理的8分钟内以98.9%的COD去除了98.3%的活性黑。

更新日期:2020-11-12
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