Japanese Journal of Applied Physics ( IF 1.5 ) Pub Date : 2020-11-05 , DOI: 10.35848/1347-4065/abc458 Yuto Kusaka 1 , Hiroyuki Fukushima 2 , Daiki Shiratori 2 , Yuma Takebuchi 2 , Kenta Igashira 2 , Daisuke Nakauchi 2 , Takumi Kato 2 , Noriaki Kawaguchi 2 , Takayuki Yanagida 2
The Ce-substituted (Ce x , Pr1-x )2Si2O7 bulk single crystals were synthesized by the floating zone method, and their photoluminescence (PL) and scintillation properties were evaluated. The X-ray diffraction patterns showed that all the synthesized samples were a single-phase of monoclinic Pr2Si2O7. In PL and scintillation, an emission peak was observed at around 370–390nm due to the 5d–4f transitions of Ce3+. In pulse height spectra, the scintillation light yield was ∼400phMeV−1 in the 99% Ce-substituted sample. The 99% Ce-substituted sample showed the highest scintillation light yield among the present samples.
中文翻译:
Ce取代的Pr 2 Si 2 O 7晶体闪烁体的光致发光和闪烁特性
通过浮区法合成了Ce取代的(Ce x,Pr 1- x)2 Si 2 O 7块状单晶,并对其光致发光(PL)和闪烁特性进行了评估。X射线衍射图谱表明,所有合成样品均为单斜晶Pr 2 Si 2 O 7单相。在PL和闪烁中,由于Ce 3+的5d-4f跃迁,在370-390nm附近观察到一个发射峰。在脉冲高度光谱中,闪烁光的产量约为400phMeV -1 在99%Ce取代的样品中 在本样品中,99%Ce取代的样品显示出最高的闪烁光产率。