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Hierarchical design of waterproof, highly sensitive, and wearable sensing electronics based on MXene-reinforced durable cotton fabrics
Chemical Engineering Journal ( IF 13.3 ) Pub Date : 2020-10-16 , DOI: 10.1016/j.cej.2020.127363
Shuang Wang , Xiaosheng Du , Yaofa Luo , Shiyu Lin , Mi Zhou , Zongliang Du , Xu Cheng , Haibo Wang

Superhydrophobic wearable textile electronics are of great promising devices due to their broad application in healthcare monitoring and artificial intelligence, etc. MXenes, the emerging two‐dimensional (2D) carbides and carbonitrides, are ideal candidates for fabricating wearable electronic devices. However, in an effort to maintain its highly conductive and long-term stability of cotton fabrics under harsh condition, it is an imperative demand to prepare superhydrophobic MXenes-textile sensor. Herein, a waterproof, highly sensitive, and wearable multi-mode sensor was successfully fabricated by the construction of 2D MXene nanosheets and zero-dimension (0D) silicon nanoparticles (SiNPs) onto a cotton fibers substrate (MX@SiNPs cotton). The as-cultivated MX@SiNPs cotton exhibited an integration of high-performance sensing toward pression, bending, and torsion, superior sensitivity (S1 = 12.23 kPa−1), a stable response under press-relaxing cycles, and broad sensing ranges (pressure: 8.8 Pa – 70 kPa, bending: 0 – 180°, torsion: 0 – 628 rad m−1). By virtue of its hierarchical structure and low surface energy of the SiNPs layer, the MXenes-textile sensor can maintain intrinsic conductivity under wet and corrosive conditions. The waterproof and highly sensitive MXene-reinforced cotton fabrics lay a basis for the broad-range application and large-scale preparation of the sensor and prolong its service life.



中文翻译:

基于MXene增强的耐用棉织物的防水,高灵敏度,可穿戴传感电子设备的分层设计

超疏水可穿戴纺织电子产品由于其在医疗保健监控和人工智能等领域的广泛应用而成为很有前途的设备。MXenes(新兴的二维(2D)碳化物和碳氮化物)是制造可穿戴电子设备的理想选择。然而,为了在恶劣条件下保持其高导电性和棉织物的长期稳定性,迫切需要制备超疏水的MXenes-纺织品传感器。在此,通过将2D MXene纳米片和零维(0D)硅纳米粒子(SiNPs)构造到棉纤维基材(MX @ SiNPs棉)上,成功地制造了防水,高灵敏且可穿戴的多模式传感器。耕种的MX @ SiNPs棉表现出对压迫,弯曲,S 1 = 12.23 kPa -1),在压力松弛的循环下具有稳定的响应,并且感应范围广(压力:8.8 Pa – 70 kPa,弯曲度:0 – 180°,扭转度:0 – 628 rad m -1)。由于其分层结构和SiNPs层的低表面能,MXenes纺织传感器可以在潮湿和腐蚀性条件下保持固有的电导率。防水且高度敏感的MXene增强棉织物为传感器的广泛应用和大规模制备奠定了基础,并延长了传感器的使用寿命。

更新日期:2020-10-16
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