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The effect of air exposure on device performance of flexible C8-BTBT organic thin-film transistors with hygroscopic insulators
Science China Materials ( IF 6.8 ) Pub Date : 2020-10-13 , DOI: 10.1007/s40843-020-1489-6
Pengshan Xie , Tianjiao Liu , Pei He , Guozhang Dai , Jie Jiang , Jia Sun , Junliang Yang

Organic thin film transistors (OTFTs) are normally sensitive to ambient conditions and show performance degradation in air. On the contrary, the performance of flexible 2,7-dioctyl[1] benzothieno [3,2-b][1]benzothiophene (C8-BTBT) OTFTs using cross-linked polymer layer, poly(4-vinyl-phenol)-4,4′-(hexafluoroisopropylidene) diphthalic anhydride (PVP-HDA), as the dielectric layer can be improved in air conditions with 40% relative humidity. Under soaking in air with 40% relative humidity, the electrical behavior, surface morphology, and contact angle of the flexible C8-BTBT OTFTs using PVP-HAD as dielectric layer with three different thicknesses were investigated. It is found that, when the devices with 375 nm-thick PVP-HDA films are placed in 40% relative humidity air conditions for 6 h, the corrected average mobility (μ) can increase from 3.2 to 5.1 cm2 V−1 s−1. Furthermore, the average threshold voltage (Vth) changes from −12.4 to −9.3 V while keeping a constant ratio of Ion/Ioff = 104. These results indicate that the flexible C8-BTBT OTFTs with PVP-HDA dielectric layer exhibit interesting application prospects.



中文翻译:

暴露于空气对带有吸湿绝缘体的柔性C8-BTBT有机薄膜晶体管的器件性能的影响

有机薄膜晶体管(OTFT)通常对环境条件敏感,并且在空气中表现出性能下降。相反,柔性2,7-二辛基[1]苯并噻吩并[3,2- b使用交联聚合物层,聚(4-乙烯基苯酚)-4,4'-(六氟异亚丙基)二邻苯二甲酸酐(PVP-HDA)作为介电层的] [1]苯并噻吩(C8-BTBT)OTFT在相对湿度为40%的空气条件下。在相对湿度为40%的空气中浸泡的情况下,研究了使用PVP-HAD作为三种不同厚度的电介质层的柔性C8-BTBT OTFT的电学性能,表面形态和接触角。据发现,当用375纳米厚的PVP-HDA膜中的设备被放置在相对湿度40%空气条件下6小时,经校正的平均迁移率(μ)可从3.2至5.1厘米增加2 V -1小号- 1。此外,平均阈值电压(V th)从-12.4变为-9.3 V,同时保持I on / I off = 10 4的恒定比率。这些结果表明,具有PVP-HDA介电层的柔性C8-BTBT OTFT表现出有趣的应用前景。

更新日期:2020-10-17
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