Graphdiyne‐Supported Atomic Catalysts: Synthesis and Applications,ChemPlusChem

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Graphdiyne‐Supported Atomic Catalysts: Synthesis and Applications
ChemPlusChem ( IF 3.0 ) Pub Date : 2020-10-14 , DOI: 10.1002/cplu.202000631
Xiaonan Kan ₁ , Chunyan Fan ₁ , Chenyu Wu ₂ , Chong Sun ₁ , Zhibo Li _{1,

3} , Yingjie Zhao ₁

Affiliation

Graphdiyne (GDY) has been ideal candidate support for atomic catalysts (ACs) due to its unique conjugated two‐dimensional (2D) structure comprising both sp‐ and sp²‐hybrid carbon atoms. ACs/GDY can display excellent catalytic ability and high selectivity, emerging as a cutting‐edge research area in the past few years. Recently, a growing body of work has been done in ACs/GDY, ranging from screening appropriate combinations theoretically, continuous improvement to prepare few‐layered GDY to meet the critical challenge in this area, and successfully fabricating ACs/GDY in facile way. This Minireview briefly introduces recent advanced progress in this field, including the synthetic method for both thin GDY film and ACs/GDY, as well as theoretical analysis of different ACs/GDY systems, characterization, and applications. In the end, the challenges and further opportunities of ACs/GDY are summarized and proposed. It is hoped that this article brings new insights into the current study of ACs/GDY and promotes better development in this area.

中文翻译：

Graphdiyne支持的原子催化剂：合成与应用

Graphdiyne（GDY）由于其独特的同时包含sp ²和sp ^2的共轭二维（2D）结构，已成为原子催化剂（AC）的理想候选载体。杂化碳原子。ACs / GDY具有出色的催化能力和高选择性，在过去几年中已成为前沿研究领域。最近，ACs / GDY的工作量不断增加，从理论上筛选适当的组合，不断改进以制备多层GDY以满足该领域的关键挑战，到成功地以容易的方式制造ACs / GDY都在不断发展。本Minireview简要介绍了该领域的最新进展，包括用于GDY薄膜和ACs / GDY的合成方法，以及不同ACs / GDY系统的理论分析，特性和应用。最后，总结并提出了AC / GDY的挑战和进一步的机会。

更新日期：2020-12-02

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