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Thermal Properties of the Quaternary Chalcogenide BaCdSnSe4
Physica Status Solidi-Rapid Research Letters ( IF 2.5 ) Pub Date : 2020-10-06 , DOI: 10.1002/pssr.202000363
Wilarachchige D. C. B. Gunatilleke 1 , Noha Alzahrani 1 , Andrew F. May 2 , Hsin Wang 2 , George S. Nolas 1
Affiliation  

The fields of nonlinear optics, photovoltaics, and thermoelectrics have been strongly impacted by materials research, and quaternary chalcogenides are one general class of materials that has recently generated strong interest. An understanding of the thermal properties is paramount in these and other applications of interest. The thermal properties of BaCdSnSe4, a quaternary chalcogenide that is of interest for applications in nonlinear optics, are reported. Specifically, the thermal conductivity over a large temperature range and heat capacity are evaluated in light of the structural features of this material. Low thermal conductivity results from the complex unit cell as well as local dynamic disorder from Cd in the CdSe4 tetrahedra in the crystal structure. The results and analyses reported herein are presented to enhance the fundamental understanding of the thermal properties of these materials, and can be related and applied to other quaternary chalcogenides that are of interest for energy‐related applications.

中文翻译:

第四级硫族化物BaCdSnSe4的热学性质

非线性光学,光伏和热电领域受到材料研究的强烈影响,季硫族化物是近来引起人们极大兴趣的一类通用材料。在这些和其他感兴趣的应用中,对热性能的了解至关重要。据报道,BaCdSnSe 4是一种季铵硫属元素,在非线性光学中非常重要,其热学性质已得到报道。具体地,根据该材料的结构特征来评估在较大温度范围内的热导率和热容量。复杂的晶胞导致低热导率,以及CdSe 4中Cd引起的局部动态紊乱四面体的晶体结构。此处介绍的结果和分析旨在增强对这些材料的热性能的基本了解,并且可以与能源相关应用感兴趣的其他季铵硫属元素相关并应用。
更新日期:2020-12-01
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