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Band alignment transition from type I to type II in GaAs / AlxGa1-x As quantum ring
Physica E: Low-dimensional Systems and Nanostructures ( IF 2.9 ) Pub Date : 2020-09-30 , DOI: 10.1016/j.physe.2020.114476
Rihab Sellami , Afef Ben Mansour , Mohamed Souhail Kehili , Adnen Melliti

We present a study of the electronic and optical properties of carriers in GaAs/AlxGa1-xAs quantum ring (QR) as a function of the aluminum concentration (x) in the barrier and the ring height (hM). We calculated the wavefunctions and the energies of the electrons and holes using the effective mass approximation. We found that the variation of x or hM, leads to a crossover, and consequently the mixing, of the electronic states of symmetry X and Γ. Then, a change from type I to type II of the GaAs/AlGaAs quantum ring occurs for x about 0.6 and hM about 1.3 nm. To present the point of type I-type II transition, we drew a color map that shows the shift of this point with x and hM. The radiative lifetime of the carriers is calculated in both type I and type II cases. In the latter case, we have taken into account the coupling between the confined electronic states of symmetry X and Γ. A value of 7 meV for the coupling potential is deduced from a comparison between our theoretical results and experimental ones. A color map showing the variation of the lifetime with x and hM was likewise drawn. Finally, these results can be exploited in several applications like solar cells.



中文翻译:

GaAs / Al x Ga 1-x As量子环中从I型到II型的能带跃迁。

我们目前对GaAs / Al x Ga 1-x As量子环(QR)中的载流子的电子和光学性质的研究,它是势垒中铝浓度(x)和环高度(h M)的函数。我们使用有效的质量近似值计算了电子和空穴的波函数和能量。我们发现x或h M的变化会导致对称X和Γ的电子状态发生交叉,从而导致混合。然后,对于大约0.6的x和大约1.3nm的h M,发生GaAs / AlGaAs量子环的从I型到II型的变化。为了显示I型到II型过渡点,我们绘制了一个颜色图,该图显示了该点在x和h M处的位移。在I型和II型情况下都计算了载流子的辐射寿命。在后一种情况下,我们考虑了对称电子X和Γ的受限电子状态之间的耦合。通过将我们的理论结果与实验结果进行比较,得出耦合电位的值为7 meV。同样绘制了显示寿命随x和h M变化的色图。最后,这些结果可以在太阳能电池等多种应用中得到利用。

更新日期:2020-10-06
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