Oxidation of Ammonia with Molecular Complexes,Journal of the American Chemical Society

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Oxidation of Ammonia with Molecular Complexes
Journal of the American Chemical Society ( IF 14.4 ) Pub Date : 2020-09-25 , DOI: 10.1021/jacs.0c08269
Peter L. Dunn ₁ , Brian J. Cook ₁ , Samantha I. Johnson ₁ , Aaron M. Appel ₁ , R. Morris Bullock ₁

Affiliation

Oxidation of ammonia by molecular complexes is a burgeon-ing area of research, with critical scientific challenges that must be addressed. A fundamental understanding of individu-al reactions steps is needed, particularly for cleavage of N-H bonds and formation of N-N bonds. This perspective evaluates the challenges of designing molecular catalysts for oxidation of ammonia, and highlights recent key contributions to realiz-ing the goals of viable energy storage and retrieval based on the N-H bonds of ammonia in a carbon-free energy cycle.

中文翻译：

用分子复合物氧化氨

通过分子复合物氧化氨是一个新兴的研究领域，必须解决关键的科学挑战。需要对各个反应步骤有基本的了解，特别是对于 NH 键的裂解和 NN 键的形成。这个观点评估了设计用于氨氧化的分子催化剂的挑战，并强调了最近在无碳能源循环中实现基于氨的 NH 键的可行能量存储和回收目标的关键贡献。

更新日期：2020-09-25

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