Synthesis of Complex Molecular Systems—The Foreseen Role of Organic Chemists,ACS Central Science

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Synthesis of Complex Molecular Systems—The Foreseen Role of Organic Chemists
ACS Central Science ( IF 12.7 ) Pub Date : 2020-09-25 , DOI: 10.1021/acscentsci.0c00974
Tobias Schnitzer _{1,

2} , Ghislaine Vantomme _{1,

2}

Affiliation

How to control the self-assembly of complex molecular systems is unknown. Yet, these complex molecular systems are fundamental for advances in material and biomedical sciences. A step forward is to transform one-step self-assembly into multistep synthesis involving covalent and noncovalent reactions. Key to this approach is to explore the chemical space at the frontiers of advanced covalent synthesis and supramolecular chemistry. Herein, we describe a selection of such reported cases and provide a guide for current limitations and insights for future directions. This outlook is meant to trigger collaborations between synthetic organic and supramolecular chemists, to expand the repertoire of organic syntheses working with supramolecular assemblies and thereby join forces to achieve stepwise emergence of molecular complexity in supramolecular systems.

中文翻译：

复杂分子系统的合成——有机化学家的预见作用

如何控制复杂分子系统的自组装尚不清楚。然而，这些复杂的分子系统是材料和生物医学科学进步的基础。向前迈出的一步是将一步自组装转变为涉及共价和非共价反应的多步合成。这种方法的关键是探索先进共价合成和超分子化学前沿的化学空间。在此，我们描述了精选的此类报告案例，并为当前的局限性提供了指导，并为未来的方向提供了见解。这一前景旨在引发合成有机化学家和超分子化学家之间的合作，扩大超分子组装体有机合成的范围，从而共同实现超分子系统中分子复杂性的逐步出现。

更新日期：2020-11-25

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