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Granular crystallization using CFBC ash for phosphorus removal via hydroxyapatite
Environmental Technology & Innovation ( IF 6.7 ) Pub Date : 2020-09-24 , DOI: 10.1016/j.eti.2020.101173
Hyangyoun Chang , Dongwoo Yoo , Hyunman Lim , Kwangho Ahn , Nari Park , Yeoju Jang , Jinhong Jung , Weonjae Kim

To prevent eutrophication and remove phosphorus, circulating fluidized bed combustion (CFBC) ash was utilized to elute Ca2+ and OH for hydroxyapatite (HAP) crystallization. CFBC ash was compared with the gypsum byproduct of a domestic waste incineration plant and pure CaO reagent. CFBC ash proved to be a suitable raw material to supply Ca2+ and OH for HAP crystallization. CFBC ash was reprocessed as a granular crystallization agent (GCA) to improve its applicability to non-point pollution source control. In addition, a manufacturing procedure for a GCA utilizing 4.8% blast furnace slag as a binder was developed based on durability and the ion elution rate in water. Column tests with sedimentation showed that 93% and 98% of T-P and PO4-P were removed after 12 h of settling, respectively. In on-site filtration trench tests, filtration following crystallization with a 4 h retention time achieved a 63.5% and 52.8% removal efficiency with respect to T-P and PO4-P, respectively. After operation for 13 d, an increase in porosity with pore distribution on the surface of the GCA was observed. Through their long-term on-site operation, crystallization-filtration trenches using GCA provide an effective alternative process for the management of agricultural non-point source pollution.



中文翻译:

使用CFBC灰进行颗粒结晶以通过羟基磷灰石去除磷

为防止富营养化并去除磷,利用循环流化床燃烧(CFBC)灰分洗脱Ca 2+和OH-用于羟基磷灰石(HAP)结晶。将CFBC灰与生活垃圾焚烧厂的石膏副产品和纯CaO试剂进行了比较。CFBC灰被证明是供应Ca 2+和OH的合适原料-用于HAP结晶。CFBC灰作为颗粒结晶剂(GCA)被重新处理,以提高其在面源污染控制中的适用性。另外,基于耐久性和水中的离子洗脱率,开发了利用4.8%高炉矿渣作为粘合剂的GCA的制造方法。沉降沉淀柱试验表明,沉降12 h后分别除去了TP和PO 4 -P的93%和98%。在现场过滤沟槽测试中,结晶后的过滤(保留时间为4小时)相对于TP和PO 4达到63.5%和52.8%的去除效率-P分别。运转13 d后,观察到GCA表面孔隙度随孔隙分布而增加。通过长期的现场操作,使用GCA的结晶过滤沟渠为管理农业面源污染提供了有效的替代方法。

更新日期:2020-09-24
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