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Rational structural design and manipulation advance SnSe thermoelectrics
Materials Horizons ( IF 12.2 ) Pub Date : 2020-08-04 , DOI: 10.1039/d0mh00954g
Xiao-Lei Shi 1, 2, 3, 4, 5 , Wen-Yi Chen 4, 5, 6, 7 , Xinyong Tao 8, 9, 10, 11 , Jin Zou 4, 5, 6, 7, 12 , Zhi-Gang Chen 1, 2, 3, 4, 5
Affiliation  

Thermoelectrics can directly harvest electricity from waste heat through the Seebeck effect; therefore, their use has been regarded as an eco-friendly and sustainable solution to alleviate the pressure due to fossil fuel consumption and environmental pollution. Rational structural manipulation is critical to improving the thermoelectric performance of materials, and a timely review is required to summarize the recent progress in novel structural design for thermoelectrics. In this review, taking SnSe as a typical example and combined with other thermoelectric materials, we summarize recent advances in rational structural manipulation for thermoelectric materials, including point defects, dislocations, boundaries, nanoinclusions, and nanopores. The inherent links between syntheses, characterization, and thermoelectric properties by tailoring their structures are established. In addition, we discuss the development of nanoscale thermoelectric materials and their potential for application in flexible thermoelectric devices. This review can guide the design of high-performance thermoelectric materials.

中文翻译:

合理的结构设计和操作方式使SnSe热电学得到了发展

热电可通过塞贝克效应直接从废热中收集电力;因此,它们的使用被认为是减轻化石燃料消耗和环境污染带来的压力的一种生态友好和可持续的解决方案。合理的结构操作对于改善材料的热电性能至关重要,需要及时审查以总结热电学新型结构设计的最新进展。在本文中,以SnSe为例,并结合其他热电材料,我们总结了热电材料的合理结构操纵方面的最新进展,包括点缺陷,位错,边界,纳米夹杂物和纳米孔。合成,表征,通过调整其结构来建立热电性能。此外,我们讨论了纳米级热电材料的发展及其在柔性热电设备中的应用潜力。这篇综述可以指导高性能热电材料的设计。
更新日期:2020-08-04
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