Abstract Due to the ongoing revolution of energy production and use as well as the increasing proliferation of electronic devices, improvements of fabrication methods and materials for electrochemical energy storage devices (EESDs), such as batteries and supercapacitors, have sparked massive research interest. Recently, printing technologies have emerged as promising fabrication methods for EESDs, while newly developed printing materials have enabled a dramatic improvement of printed electrodes due to lower cost, more facile preparation, and enhanced electrochemical and mechanical properties. This review provides an overview of printing technologies for EESD fabrication and focuses primarily on graphene-based materials. We cover inkjet, aerosol-jet, screen, roll-to-roll and 3D printing methods, survey the recent literature, present illustrative examples of technical applications of printing technologies for energy storage, and describe, in detail, prepared ink formulations, printing procedures, and electrochemical performances.

中文翻译：

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基于石墨烯的超级电容器和电池的 2D 和 3D 打印：综述

摘要 由于能源生产和使用的持续革命以及电子设备的日益普及，电化学储能设备（EESD）（例如电池和超级电容器）的制造方法和材料的改进引发了广泛的研究兴趣。最近，印刷技术已成为有前途的 EESD 制造方法，而新开发的印刷材料由于成本更低、制备更容易以及电化学和机械性能增强，使得印刷电极的性能得到显着改善。本综述概述了 EESD 制造的印刷技术，主要关注基于石墨烯的材料。我们涵盖喷墨、气溶胶喷射、丝网、卷对卷和 3D 打印方法，调查最近的文献，