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A Ternary-Mixture-Based Counter Electrode for Quantum-Dot-Sensitized Solar Cells
ACS Applied Energy Materials ( IF 5.4 ) Pub Date : 2020-07-07 00:00:00 , DOI: 10.1021/acsaem.0c01177
Dan Li, Zhiqiang Fu, Qiuchen Han, Chen-Hsueh Lin, Shufang Gao, Yan Xiong, Ten-Chin Wen

A ternary mixture of carbon, copper sulfide, and cobalt sulfide was used to fabricate the counter electrode (CE) in quantum-dot-sensitized solar cells (QDSSCs). The ternary-mixture-based CE achieved much higher energy conversion efficiency than any CE based on the individual material. The mixture and the CE were investigated by photocurrent density–voltage characteristics, X-ray diffraction patterns, electrochemical impedance spectroscopy, and contour line plots. A balanced mix results in enhanced photocurrent and reduced charge transfer resistance at the interface, and this leads to optimized device performance. The highest photoelectric conversion efficiency was 3.73% at a 1:1:1 mass ratio. The efficiency was as high as 3.09% via a corresponding flexible CE.

中文翻译:

基于三元混合物的量子点敏化太阳能电池对电极

碳,硫化铜和硫化钴的三元混合物用于制造量子点敏化太阳能电池(QDSSC)中的对电极(CE)。基于三元混合物的CE的能量转换效率远高于任何基于单个材料的CE。通过光电流密度-电压特性,X射线衍射图,电化学阻抗谱和等高线图研究了混合物和CE。平衡的混合可增强光电流并降低界面处的电荷转移电阻,从而可优化器件性能。在1∶1∶1的质量比下,最高的光电转换效率为3.73%。通过相应的灵活CE,效率高达3.09%。
更新日期:2020-07-07
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