当前位置: X-MOL 学术Deep Sea Res. Part I Oceanogr. Res. Pap. › 论文详情
Our official English website, www.x-mol.net, welcomes your feedback! (Note: you will need to create a separate account there.)
210Po and 210Pb distributions during a phytoplankton bloom in the North Atlantic: Implications for POC export
Deep Sea Research Part I: Oceanographic Research Papers ( IF 2.3 ) Pub Date : 2020-07-07 , DOI: 10.1016/j.dsr.2020.103339
Evan J. Horowitz , J. Kirk Cochran , Michael P. Bacon , David J. Hirschberg

During the North Atlantic Bloom Experiment (NABE) of the Joint Global Ocean Flux Study (JGOFS), water column sampling for particulate and dissolved 210Po and 210Pb was performed four times (26 April and 4, 20, 30 May 1989) during a month-long Lagrangian time-series occupation of the NABE site, as well as one-time samplings at stations during transit to and from the site. There are few prior studies documenting short-term changes in 210Po and 210Pb profiles over the course of a phytoplankton bloom, and we interpret the profiles in terms of the classical “steady-state” (SS) approach used in most studies, as well as by using a non-steady state approach suggested by the temporal evolution of the profiles. Changes in 210Po profiles during a bloom are expectable as this radionuclide is scavenged and exported. During NABE, 210Pb profiles also displayed non-steady state, with significant increases in upper water column inventory occurring midway through the experiment. Export of 210Po from the upper 150 m using the classic “steady-state” model shows increases from 0.5 ± 8.5 dpm m−2 d−1 to 68.2 ± 4.2 dpm m−2 d−1 over the ~one-month occupation. Application of a non-steady state model, including changes in both 210Pb and 210Po profiles, gives higher 210Po export fluxes. Detailed depth profiles of particulate organic carbon (>0.8 μm) and particulate 210Po (>0.4 μm) are available from the 20 and 30 May samplings and show maxima in POC/Po at ~37 m. Applying the POC/210Po ratios at 150 m to the “steady state” 210Po fluxes yields POC export from the upper 150 m of 8.2 ± 1.5 mmol C m− 2 d−1 on 20 May and 6.0 ± 1.6 mmol C m−2 d−1 on 30 May. The non-steady state model applied to the interval 20 to 30 May yields POC export of 24.3 mmol C m−2 d−1. The non-steady state (NSS) 210Po-derived POC fluxes are comparable to, but somewhat less than, those estimated previously from 234Th/238U disequilibrium for the same time interval (37.3 and 45.0 mmol m−2 d−1, depending on the POC/Th ratio used). In comparison, POC fluxes measured with a floating sediment trap deployed at 150 m from 20 to 30 May were 11.6 mmol m−2 d−1. These results suggest that non-steady state Po-derived POC fluxes during the NABE agree well with those derived from 234Th/238U disequilibrium and agree with sediment trap fluxes within a factor of ~2. However, unlike the 234Th-POC flux proxy, non-steady stage changes in profiles of 210Pb, the precursor of 210Po, must be considered.



中文翻译:

北大西洋浮游植物开花期间的210 Po和210 Pb分布:对POC出口的影响

在联合全球海洋通量研究(JGOFS)的北大西洋布卢姆实验(NABE )期间,在1989年4月26日和4月20日,4月20日,1989年5月30日对水颗粒和溶解的210 Po和210 Pb进行了水柱采样NABE站点长达一个月的拉格朗日时间序列占用,以及往返站点期间在站点上的一次采样。先前的研究很少记录浮游植物开花过程中210 Po和210 Pb剖面的短期变化,并且我们根据大多数研究中使用的经典“稳态”(SS)方法来解释剖面,因为以及通过使用轮廓的时间演变所建议的非稳态方法。210的变化由于这种放射性核素被清除并输出,因此预计在开花期间会产生Po分布。在NABE期间,210 Pb剖面也显示出非稳态,实验中途发生的上部水柱存量显着增加。使用经典的“稳态”模型从上部150 m出口210 Po表示在一个月的使用时间内从0.5±8.5 dpm m -2 d -1增加到68.2±4.2 dpm m -2 d -1。非稳态模型的应用(包括210 Pb和210 Po剖面的变化)给出了更高的210宝出口通量。从5月20日和30日的采样中可以获得颗粒有机碳(> 0.8μm)和210 Po(> 0.4μm)颗粒的详细深度剖面图,并显示了〜37 m处POC / Po的最大值。施加POC / 210,在150米宝比到“稳定状态” 210宝通量产量POC出口从8.2±1.5毫摩尔C M上150米- 2 d -1 5月20日和6.0±1.6毫摩尔C M - 5月30日2 d -1。应用于5月20日至30日的非稳态模型将产生24.3 mmol C m -2 d -1的POC出口。非稳态(NSS)210在相同的时间间隔内(37.3和45.0 mmol m -2 d -1,取决于所使用的POC / Th比率),Po衍生的POC通量与以前从234 Th / 238 U不平衡所估算的通量可比,但略小于这些通量。。相比之下,从5月20日至30日在150 m处部署的浮动沉积物陷阱测得的POC通量为11.6 mmol m -2 d -1。这些结果表明,NABE期间非稳态Po衍生的POC通量与从234 Th / 238 U不平衡中导出的POC通量非常吻合,并且在约2倍内与沉积物捕集通量吻合。但是,与234不同必须考虑Th-POC通量代理,210 Pb(210 Po的前兆)剖面的非稳态变化。

更新日期:2020-09-12
down
wechat
bug