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Fabrication of MoS2 QDs/ZnO nanosheet 0D/2D heterojunction photocatalysts for organic dyes and gaseous heavy metal removal.
Journal of Colloid and Interface Science ( IF 9.4 ) Pub Date : 2020-07-03 , DOI: 10.1016/j.jcis.2020.06.116
Ruiqi Gang 1 , Lei Xu 1 , Yi Xia 2 , Jun Cai 3 , Libo Zhang 1 , Shixing Wang 1 , Rui Li 1
Affiliation  

In this paper, a novel 0D/2D heterojunction photocatalyst based on MoS2 QDs/ZnO nanosheets was successfully constructed by a simple two-step process, and its photocatalytic behavior for organic dyes (RhB) degradation and gaseous heavy metals (Hg) removal under ultraviolet light were studied. For the optimum 5% MoS2/ZnO photocatalyst, 95% of RhB could be removed in 50 min, and 99.8% of the gaseous mercury could be removed in 60 min. Besides, MoS2 QDs/ZnO nanosheets also exhibited excellent photocatalytic durability. The constructed 0D/2D heterojunctions could efficiently improve the separation efficiency and charge transfer of photogenerated carriers, thus improving the photocatalytic activity. Therefore, this strategy provided a new way to design bifunctional 0D/2D heterojunction photocatalysts for water treatment and air pollution.



中文翻译:

MoS2 QDs / ZnO纳米片0D / 2D异质结光催化剂的制备,用于有机染料和气态重金属的去除。

本文通过简单的两步法成功构建了基于MoS 2 QDs / ZnO纳米片的新型0D / 2D异质结光催化剂,并在光催化下降解有机染料(RhB)和去除气态重金属(Hg)的光催化行为。研究了紫外线。对于最佳的5%MoS 2 / ZnO光催化剂,可以在50分钟内除去95%的RhB,在60分钟内可以除去99.8%的气态汞。此外,MoS 2QDs / ZnO纳米片也表现出出色的光催化耐久性。构造的0D / 2D异质结可以有效提高光生载流子的分离效率和电荷转移,从而提高了光催化活性。因此,该策略为设计用于水处理和空气污染的双功能0D / 2D异质结光催化剂提供了新途径。

更新日期:2020-07-05
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