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Two-Dimensional Layered Materials: High-Efficient Electrocatalysts for Hydrogen Evolution Reaction
ACS Applied Nano Materials ( IF 5.3 ) Pub Date : 2020-06-30 , DOI: 10.1021/acsanm.0c01331
Qing Zhu 1 , Yuanju Qu 2 , Detao Liu 3 , Kar Wei Ng 1 , Hui Pan 1, 4
Affiliation  

Hydrogen production via water splitting is considered to be one of the most promising technologies in the future hydrogen economy, where the critical challenge in this technology is exploring high-efficient and cost-effective electrocatalysts. Currently, extensive works from both experimental and theoretical investigations have shown that two-dimensional (2D) layered materials can be highly energetic electrocatalysts for electrically driven hydrogen production. Herein, recent progress in 2D layered materials such as electrocatalysts, including graphene, graphitic carbon nitride, transitional-metal dichalcogenides, and MXenes for the hydrogen evolution reaction (HER) will be systematically discussed and summarized. This review provides a broad overview on a wide range of strategies to design and fabricate 2D layered materials as electrocatalysts with high-catalytic performance for HER and aims to give potential avenues for the design of catalysts for commercial applications. In addition, the key scientific issues to address the 2D layered materials as HER catalysts are highlighted, and the perspective on the future development is given at the end.

中文翻译:

二维层状材料:氢气析出反应的高效电催化剂

通过水分解制氢被认为是未来氢经济中最有前途的技术之一,该技术的关键挑战是探索高效和具有成本效益的电催化剂。当前,来自实验和理论研究的大量工作表明,二维(2D)层状材料可以是用于驱动氢生产的高能电催化剂。在此,将系统地讨论和总结2D层状材料的最新进展,例如电催化剂,包括石墨烯,石墨碳氮化物,过渡金属二卤化物和MXenes。这篇综述广泛地概述了设计和制造二维层状材料作为HER高催化性能电催化剂的各种策略,旨在为商业应用的催化剂设计提供潜在途径。此外,重点介绍了解决2D层状材料作为HER催化剂的关键科学问题,并在最后给出了对未来发展的看法。
更新日期:2020-07-24
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