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SnO2 nanoparticles-modified 3D-multilayer MoS2 nanosheets for ammonia gas sensing at room temperature
Sensors and Actuators B: Chemical ( IF 8.0 ) Pub Date : 2020-06-20 , DOI: 10.1016/j.snb.2020.128471
Wenxin Wang , Yuhua Zhen , Jiuyang Zhang , Yingda Li , Hong Zhong , Zilong Jia , Ya Xiong , Qingzhong Xue , Youguo Yan , Njud S. Alharbi , Tasawar Hayat

In this work, MoS2 nanosheets decorated with SnO2 nanoparticles were prepared via a facile two-step hydrothermal method, which possesses a proposed sensing composite structure of supporting layer/sensitive dots. The SnO2/MoS2 nanocomposites exhibited an excellent sensing response (2080.36) toward 200 ppm NH3, which was ∼27.5 times higher than that of pristine MoS2 films, a fast response/recovery time (23/1.6 s) toward 50 ppm at room temperature (22℃), and outstanding selectivity to NH3 against CH4, H2, CO, H2S, and NO2 and good repeatability. The excellent gas sensing properties could be dominated by the unique thin layers assembled flower-like structures of 2D MoS2, which foster the carrier charge transfer process and the reaction to SnO2/MoS2 and NH3. These results present the SnO2/MoS2 nanocomposites promising candidate materials for high-performance NH3 gas sensing at room temperature.



中文翻译:

SnO 2纳米粒子修饰的3D多层MoS 2纳米片,用于室温下的氨气传感

在这项工作中,通过方便的两步水热法制备了装饰有SnO 2纳米粒子的MoS 2纳米片,该方法具有拟议的支撑层/敏感点的感测复合结构。SnO 2 / MoS 2纳米复合材料对200 ppm NH 3表现出出色的感测响应(2080.36),比原始MoS 2膜高约27.5倍,对50 ppm的响应/恢复时间短(23 / 1.6 s)在室温(22℃)下,对NH 3对CH 4,H 2,CO,H 2 S和NO 2的选择性很高重复性好 优异的气体感测性能可能由2D MoS 2的独特的薄层组装花状结构主导,这促进了载流子电荷转移过程以及与SnO 2 / MoS 2和NH 3的反应。这些结果表明SnO 2 / MoS 2纳米复合材料有望在室温下用于高性能NH 3气体传感的候选材料。

更新日期:2020-07-02
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