Oxidative cascade cyclization of 2-cyano-3-arylaniline derived acrylamides with toluenes, ethers, aliphatic alcohols or simple alkanes,Organic Chemistry Frontiers

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Oxidative cascade cyclization of 2-cyano-3-arylaniline derived acrylamides with toluenes, ethers, aliphatic alcohols or simple alkanes
Organic Chemistry Frontiers ( IF 4.6 ) Pub Date : 2020-06-16 , DOI: 10.1039/d0qo00535e
Wen-Jin Xia _{1,

2,

3,

4} , Yangchun Xin _{5,

6,

7,

8} , Zhi-Wei Zhao _{1,

2,

3,

4} , Xin Chen _{1,

2,

3,

4} , Xiang-Xiang Wang _{1,

2,

3,

4} , Yi Li _{1,

2,

3,

4} , Guanlin Wang _{1,

2,

3,

4} , Ya-Min Li _{1,

2,

3,

4}

Affiliation

An oxidative radical cascade cyclization of 2-cyano-3-arylaniline derived acrylamides with hydrocarbons is described. The present reaction exhibits a wide substrate scope, and toluenes, ethers, aliphatic alcohols and simple alkanes can be employed as coupling partners, providing access to alkyl substituted pyrido[4,3,2-gh]phenanthridines.

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