Ni–Co–Cu–Mn Ferrite $$+$$ PZT ($${\hbox {PbZr}}_{0.52} {\hbox {Ti}}_{0.48} {\hbox {O}}_{3}$$) ferroelectric: composite thick films were prepared by the screen-printing method. The normal XRD and the low glancing angle XRD confirm the presence of both phases in the composite thick films. Back-scattered SEM shows 0-3 and 3-3 types of connectivity. The magnetic ordering of the ferrite phase was confirmed from $$M\hbox {--}H$$ hysteresis loop whereas the electric ordering of the ferroelectric phase was confirmed from $$P\hbox {--}E$$ hysteresis curve. Various measurable parameters from the loop were studied as a function of the mole percent of constituent phases. PUND (positive up negative down) analysis was done to determine the resultant polarisation contributed by the participating phases in the composites. Dielectric and magnetoelectric (ME) measurements were analysed in the light of PUND measured data.

中文翻译：

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Ni-Co-Cu-Mn 铁氧体 $$+$$ PZT 复合厚膜的结构、磁性和电学性能

Ni–Co–Cu–Mn 铁氧体 $$+$$ PZT ($${\hbox {PbZr}}_{0.52} {\hbox {Ti}}_{0.48} {\hbox {O}}_{3} $$) 铁电体：通过丝网印刷方法制备复合厚膜。正常 XRD 和低掠射角 XRD 证实了复合厚膜中两种相的存在。背向散射 SEM 显示 0-3 和 3-3 类型的连接。铁氧体相的磁序由 $$M\hbox {--}H$$ 磁滞回线证实，而铁电相的电序由 $$P\hbox {--}E$$ 磁滞曲线证实。作为组成相摩尔百分比的函数，研究了来自回路的各种可测量参数。进行 PUND（正上负下）分析以确定由复合材料中的参与相贡献的合成极化。