Manganese and Vanadium Oxide Cathodes for Aqueous Rechargeable Zinc-Ion Batteries: A Focused View on Performance, Mechanism, and Developments,ACS Energy Letters

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Manganese and Vanadium Oxide Cathodes for Aqueous Rechargeable Zinc-Ion Batteries: A Focused View on Performance, Mechanism, and Developments
ACS Energy Letters ( IF 19.3 ) Pub Date : 2020-06-09 , DOI: 10.1021/acsenergylett.0c00740
Vinod Mathew ₁ , Balaji Sambandam ₁ , Seokhun Kim ₁ , Sungjin Kim ₁ , Sohyun Park ₁ , Seulgi Lee ₁ , Muhammad Hilmy Alfaruqi ₁ , Vaiyapuri Soundharrajan ₁ , Saiful Islam ₁ , Dimas Yunianto Putro ₁ , Jang-Yeon Hwang ₁ , Yang-Kook Sun ₂ , Jaekook Kim ₁

Affiliation

The development of new battery technologies requires them to be well-established given the competition from lithium ion batteries (LIBs), a well-commercialized technology, and the merits should surpass other available technologies’ characteristics for battery applications. Aqueous rechargeable zinc ion batteries (ARZIBs) represent a budding technology that can challenge LIBs with respect to electrochemical features because of the safety, low cost, high energy density, long cycle life, high-volume density, and stable water-compatible features of the metal zinc anode. Research on ARZIBs utilizing mild acidic electrolytes is focused on developing cathode materials with complete utilization of their electro-active materials. This progress is, however, hindered by persistent issues and consequences of divergent electrochemical mechanisms, unwanted side reactions, and unresolved proton insertion phenomena, thereby challenging ARZIB commercialization for large-scale energy storage applications. Herein, we broadly review two important cathodes, manganese and vanadium oxides, that are witnessing rapid progress toward developing state-of-the-art ARZIB cathodes.

中文翻译：

水性可充电锌离子电池的锰和钒氧化物阴极：性能，机理和发展的集中观点

鉴于锂离子电池（LIB）是一项商业化良好的技术，新电池技术的发展要求它们建立良好的基础，其优点应超过电池应用中其他可用技术的特征。水性可充电锌离子电池（ARZIBs）代表了一项崭新的技术，因为其安全性，低成本，高能量密度，长循环寿命，高体积密度以及稳定的与水相容的特性，可在电化学特性方面挑战LIB。金属锌阳极。利用温和的酸性电解质对ARZIBs进行研究的重点是开发完全利用其电活性材料的阴极材料。但是，持续的问题和不同电化学机制的后果阻碍了这一进展，有害的副反应和未解决的质子插入现象，从而挑战了ARZIB在大规模储能应用中的商业化应用。在此，我们广泛地回顾了两个重要的阴极，即锰和钒氧化物，它们正朝着开发最新的ARZIB阴极发展。

更新日期：2020-07-10

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