当前位置: X-MOL 学术Int. J. Greenh. Gas. Con. › 论文详情
Our official English website, www.x-mol.net, welcomes your feedback! (Note: you will need to create a separate account there.)
The correlation between pO2 and pCO2 as a chemical marker for detection of offshore CO2 leakage
International Journal of Greenhouse Gas Control ( IF 4.6 ) Pub Date : 2020-06-07 , DOI: 10.1016/j.ijggc.2020.103085
Christian Totland , Espen Eek , Ann E.A. Blomberg , Ivar-Kristian Waarum , Peer Fietzek , Axel Walta

A controlled CO2 release experiment was carried out in order to mimic unintended leakage of geologically stored CO2, and to study methods for detecting these leak events. The experiment was carried out at 60 m depth in the Oslo Fjord over the course of one month. During the simulated leak events, the water chemistry was monitored by sensors mounted on stationary templates located 10 and 22 m horizontally from the source, as well as sensors mounted on an Autonomous Underwater Vehicle (AUV). During baseline conditions (no CO2 release), we observe a strong biogenic correlation between O2 and CO2. This correlation is lacking during CO2 releases, indicating that the CO2-O2 correlation can be used as a marker for CO2 leakage. The same deviations were not initially detected by the CO2 sensor mounted on the AUV due to the longer response time of membrane-based CO2 sensors. However, by applying response time correction in the post-processing of the AUV CO2 data, the generated CO2 plume was detected. Moreover, the plume was clearly detected by the AUV using the faster responding pH sensors, where the correlation with O2 again could be used to confirm the anomaly.



中文翻译:

pO 2和pCO 2作为检测海上CO 2泄漏的化学标记物之间的相关性

为了模拟地质存储的CO 2的意外泄漏,并研究检测这些泄漏事件的方法,进行了受控的CO 2释放实验。该实验在一个月的时间里于奥斯陆峡湾的60 m深度进行。在模拟泄漏事件期间,通过安装在距水源水平10和22 m的固定模板上的传感器以及安装在自动水下航行器(AUV)上的传感器对水化学进行监测。在基线条件下(无CO 2释放),我们观察到O 2和CO 2之间存在很强的生物相关性。在CO 2释放期间缺乏这种相关性,表明CO 2-O 2相关性可以用作CO 2泄漏的标记。由于基于膜的CO 2传感器的响应时间较长,最初安装在AUV上的CO 2传感器未检测到相同的偏差。但是,通过在AUV CO 2数据的后处理中应用响应时间校正,可以检测到生成的CO 2羽流。此外,AUV使用响应速度更快的pH传感器可以清楚地检测出羽流,其中与O 2的相关性可再次用于确认异常。

更新日期:2020-06-07
down
wechat
bug