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Dynamic depth distribution of cesium-133 near soil surfaces in packed soils under multiple simulated rains
Catena ( IF 5.4 ) Pub Date : 2020-05-30 , DOI: 10.1016/j.catena.2020.104710
X.C. (John) Zhang

Various 137Cs conversion models have been used to predict soil erosion. A knowledge of the initial distribution of 137Cs is vital to improve soil loss prediction. The objectives were to (1) characterize the dynamic distributions of 133Cs near the soil surfaces in multiple rains spiked with 133Cs using a rainfall simulator, and (2) further estimate the relaxation mass depth (H) for use in an improved 137Cs mass balance model. Three silt loam soils were packed to soil boxes (1 × 0.5 × 0.1 m) and rained on at 30 mm h−1 and 10% slope in five consecutive rains. Soil cores (62.5 mm i.d.) were taken following each rain and were sectioned in the 1–10-mm intervals. Event runoff and sediment were collected. Cs+ was extracted with an NH4OAc method using a centrifuge procedure and analyzed with Inductively Coupled Plasma-Mass Spectrometer. The results showed initial Cs distributions near the soil surfaces were approximately exponential, and the mean H value could adequately characterize the initial Cs distributions for each soil for any sequence of rains. The averaged H values were 0.338, 0.304, and 0.354 g cm−2 for the three soils, equivalent to the soil depths of 2.76, 2.20, and 2.58 mm, indicating that majority of Cs was distributed within the top 3-mm depth. Cs+ was strongly adsorbed by the soils as indicated by the large Kd values of >32.6 L kg−1, showing the limited mobility of the freshly deposited Cs+ in the soils. Better H estimation should lead to more accurate soil loss prediction using the improved Cs mass balance model.



中文翻译:

多次模拟降雨下填充土壤中铯133在土壤表层的动态深度分布

各种137 Cs转换模型已用于预测土壤侵蚀。了解137 Cs的初始分布对于改善土壤流失预测至关重要。目的是(1)使用降雨模拟器描述在多次降雨中以133 Cs加标的土壤表面中133 Cs的动态分布,以及(2)进一步估算弛豫质量深度(H),以用于改进的137 Cs质量平衡模型。将三种淤泥质壤土包装到土箱(1×0.5×0.1 m)中,并在30 mm h -1上降雨连续五次降雨的坡度为10%。每次下雨后取土芯(内径62.5毫米),并以1-10毫米的间隔切开。收集事件径流和沉积物。使用NH 4 OAc方法通过离心程序提取Cs +,并使用电感耦合等离子体质谱仪进行分析。结果表明,土壤表面附近的初始Cs分布近似呈指数分布,并且平均H值可以充分表征任何降雨序列下每种土壤的初始Cs分布。平均H值为0.338、0.304和0.354 g cm -2对于这三种土壤,其土壤深度分别为2.76、2.20和2.58 mm,这表明大多数Cs分布在顶部3 mm深度内。如> 32.6 L kg -1的大K d值所示,Cs +被土壤强烈吸附,表明新鲜沉积的Cs +在土壤中的活动性有限。使用改良的Cs质量平衡模型,更好的H估计将导致更准确的土壤流失预测。

更新日期:2020-05-30
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