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Yearlong first measurements of black carbon in the western Indian Himalaya: Influences of meteorology and fire emissions
Atmospheric Pollution Research ( IF 3.9 ) Pub Date : 2020-04-24 , DOI: 10.1016/j.apr.2020.04.015
Chhavi P. Pandey , Jaydeep Singh , Vijay K. Soni , Narendra Singh

Measurements of equivalent black carbon (EBC) aerosols are presented for the first time from a high-altitude station Ranichauri (30°18′ N, 78°24′ E; 2200 m amsl) in the lesser Himalaya during January-December 2016. The influences of meteorology, fire emissions and transport, on [EBC] variations have been investigated here. The daily mean values of [EBC] are observed to vary from 0.04 ± 0.03 μgm−3 to 7.83 ± 2.66 μgm−3 with peak during April. A significant enhancement in [EBC] is observed towards the end of April, reaching the levels as high as 23.95 μgm−3 and attributed to fire emissions. Diurnal variations are suppressed with typically lower [EBC] levels during the summer monsoon (0.42 ± 0.25 μg m−3 in July) due to the transport of marine air mass and scavenging. On a seasonal basis, the average [EBC] levels are found to be higher during winter (2.72 ± 1.86 μgm−3) and pre-monsoon (2.56 ± 1.80 μg m−3), and lowest during the summer monsoon (0.89 ± 01.03 μg m−3).Our measurements in conjunction with the analysis of model meteorology (Era Interim reanalysis) show profound effects of boundary layer dynamics on EBC concentrations. Wintertime [EBC] maximum is suggested to be due to confinement of regional anthropogenic emissions in shallow boundary layer. In addition, transport from the North-West, and Western regions, characterized by wood-burning and fossil fuel combustion, also affected [EBC] the variations here, except during the summer monsoon.



中文翻译:

印度西部喜马拉雅山一年以来首次对黑碳进行测量:气象学和火灾排放的影响

2016年1月至12月,首次在小喜马拉雅山的高海拔站Ranichauri(北纬30°18′N,东经78°24′E; 2200 m amsl)测量了等效的黑碳(EBC)气溶胶。此处已经研究了气象,火灾排放和运输对[EBC]变化的影响。[EBC]的每日平均值都观察到变化从0.04±0.03μgm -3到7.83±2.66μgm -3四月期间与峰。在[EBC]甲显著增强朝向四月底观察到,在到达水平高达23.95μgm -3和归因于火的排放。在夏季季风期间,通常以较低的[EBC]水平抑制昼夜变化(0.42±0.25μgm -3在七月)由于海洋气团的运输和清除。按季节,平均[EBC]水平被发现是在冬季较高(2.72±1.86μgm -3)和预季风(2.56±1.80微克米-3),和夏季风期间最低(0.89±01.03 μgm -3)。我们的测量与模型气象分析(时代中期再分析)一起显示了边界层动力学对EBC浓度的深远影响。冬季[EBC]最大值建议归因于浅边界层区域人为排放的限制。此外,以西北地区和西部地区为特征的运输(以木材燃烧和化石燃料燃烧为特征)也影响了[EBC]变化,除了夏季风。

更新日期:2020-04-24
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