The fluid synergy between experimentalists and theoreticians has, for decades, led to a deeper understanding of the processes that govern single‐molecule magnets. This approach has allowed for the establishment of proven design criteria for the control of magnetic properties through molecular architecture and the development of new magnetic measurement techniques and innovative computational methodologies. Here, we give an account of the experimental and theoretical joint endeavor carried out as part of the synthesis group led by David Mills and the computational/theoretical team led by Nicholas Chilton, together with colleagues in synthetic f‐element chemistry and magnetism at the University of Manchester. In addition, we provide a personal perspective on collaborative work in molecular magnetism and how such collaborations are essential for advancing the field further.

中文翻译：

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引人入胜的吸引力：分子磁性领域的合作与反馈

数十年来，实验学家和理论家之间的流体协同作用使人们对控制单分子磁体的过程有了更深入的了解。这种方法允许建立通过分子结构控制磁性能的可靠设计标准，并开发新的磁测量技术和创新的计算方法。在这里，我们介绍了由戴维·米尔斯（David Mills）和尼古拉斯·奇尔顿（Nicholas Chilton）领导的计算/理论小组，以及大学的合成元素化学和磁性领域的同事组成的合成小组进行的实验和理论上的共同努力。曼彻斯特 此外，